ENTRY O2602 20240229 O260200000001 SUBENT O2602001 20240229 20260228 O260200100001 BIB 10 20 O260200100002 TITLE Study of thulium-167 cyclotron production: a potential O260200100003 medically-relevant radionuclide O260200100004 AUTHOR (E.Renaldin, G.Dellepiane, S.Braccini, A.Sommerhalder, O260200100005 H.Zhang, N.P.Van Der Meulen, R.Eichler, Z.Talip) O260200100006 INSTITUTE (2SWTPSI,2SWTUBE) O260200100007 REFERENCE (J,FRCH,2,1288588,2024) O260200100008 FACILITY (CYCLO,2SWTUBE) 18-MeV medical cyclotron O260200100009 DETECTOR (HPGE) O260200100010 METHOD (ACTIV,BCINT) The irradiation time (13-18 min) and O260200100011 proton current < 10 nA O260200100012 ERR-ANALYS (ERR-T) Total uncertainty are due: O260200100013 (ERR-1,,1.) target mass (<1%) O260200100014 (ERR-2) integrated current (1%) O260200100015 (ERR-3) beam flatness (5%) O260200100016 (ERR-4,,10.) detection efficiency (<10%) O260200100017 (ERR-5,,5.) statistical error due to O260200100018 radioactive decay (<5%) O260200100019 (ERR-6) half-life (~0.2%) O260200100020 STATUS (APRVD) Approved by Z.Talip (2024-03-07) O260200100021 HISTORY (20240229C) VT O260200100022 ENDBIB 20 0 O260200100023 COMMON 3 3 O260200100024 ERR-2 ERR-3 ERR-6 O260200100025 PER-CENT PER-CENT PER-CENT O260200100026 1. 5. 0.2 O260200100027 ENDCOMMON 3 0 O260200100028 ENDSUBENT 27 0 O260200199999 SUBENT O2602002 20240229 20260228 O260200200001 BIB 6 18 O260200200002 REACTION ((68-ER-167(P,3N)69-TM-165,,SIG)+ O260200200003 (68-ER-166(P,2N)69-TM-165,,SIG,,FCT)) O260200200004 FCT=0.96/96.3 O260200200005 DECAY-DATA (69-TM-165,30.06HR,DG,242.9,0.355) O260200200006 SAMPLE The enriched 167ErO3 sample with the following isotopicO260200200007 composition: O260200200008 Isotope: 162Er 164Er 166Er 167Er 168Er 170Er O260200200009 Abundance: <0.01 0.01 0.96 96.3 2.57 0.16 O260200200010 (68-ER-166,ENR=0.0096) O260200200011 (68-ER-167,ENR=0.963) O260200200012 COMMENT By compiler: Results reported as 167Er(p,x)165Tm O260200200013 compiled as sum of contributing reactions considering O260200200014 the reaction thresholds: O260200200015 165Tm production: Reaction; E threshold O260200200016 166Er+p; 11.0 MeV O260200200017 167Er+p; 17.4 MeV O260200200018 ERR-ANALYS (ERR-7) absolute gamma-ray intensity (5%) O260200200019 STATUS (TABLE,,E.Renaldin+,J,FRCH,2,1288588,2024) Table 3 O260200200020 ENDBIB 18 0 O260200200021 COMMON 1 3 O260200200022 ERR-7 O260200200023 PER-CENT O260200200024 5. O260200200025 ENDCOMMON 3 0 O260200200026 DATA 4 9 O260200200027 EN EN-ERR DATA ERR-T O260200200028 MEV MEV MB MB O260200200029 11.5 0.4 1.31 0.53 O260200200030 13.0 0.4 4.87 0.83 O260200200031 14.1 0.4 5.65 0.84 O260200200032 14.5 0.4 5.59 0.59 O260200200033 15.2 0.4 6.53 1.09 O260200200034 15.8 0.4 6.81 0.66 O260200200035 16.5 0.4 11.3 1.5 O260200200036 17.1 0.4 12.9 1.4 O260200200037 18.2 0.4 26.5 1.9 O260200200038 ENDDATA 11 0 O260200200039 ENDSUBENT 38 0 O260200299999 SUBENT O2602003 20240229 20260228 O260200300001 BIB 6 18 O260200300002 REACTION ((68-ER-167(P,2N)69-TM-166,,SIG)+ O260200300003 (68-ER-166(P,N)69-TM-166,,SIG,,FCT)) O260200300004 FCT=0.96/96.3 O260200300005 DECAY-DATA (69-TM-166-G,7.70HR,DG,778.8,0.191) O260200300006 SAMPLE The enriched 167ErO3 sample with the following isotopicO260200300007 composition: O260200300008 Isotope: 162Er 164Er 166Er 167Er 168Er 170Er O260200300009 Abundance: <0.01 0.01 0.96 96.3 2.57 0.16 O260200300010 (68-ER-166,ENR=0.0096) O260200300011 (68-ER-167,ENR=0.963) O260200300012 COMMENT By compiler: Results reported as 167Er(p,x)166Tm O260200300013 compiled as sum of contributing reactions considering O260200300014 the reaction thresholds: O260200300015 166Tm production: Reaction; E threshold O260200300016 166Er+p; 3.8 MeV O260200300017 167Er+p; 10.3 MeV O260200300018 ERR-ANALYS (ERR-7) absolute gamma-ray intensity (5%) O260200300019 STATUS (TABLE,,E.Renaldin+,J,FRCH,2,1288588,2024) Table 3 O260200300020 ENDBIB 18 0 O260200300021 COMMON 1 3 O260200300022 ERR-7 O260200300023 PER-CENT O260200300024 5. O260200300025 ENDCOMMON 3 0 O260200300026 DATA 4 14 O260200300027 EN EN-ERR DATA ERR-T O260200300028 MEV MEV MB MB O260200300029 8.7 0.4 1.26 0.11 O260200300030 9.7 0.4 2.39 0.30 O260200300031 10.4 0.4 8.36 1.00 O260200300032 11.1 0.4 80.4 7.0 O260200300033 11.5 0.4 138. 12. O260200300034 12.1 0.4 266. 24. O260200300035 13.0 0.4 350. 30. O260200300036 14.1 0.4 534. 33. O260200300037 14.5 0.4 614. 43. O260200300038 15.2 0.4 632. 39. O260200300039 15.8 0.4 684. 46. O260200300040 16.5 0.4 740. 46. O260200300041 17.1 0.4 729. 63. O260200300042 18.2 0.4 800. 50. O260200300043 ENDDATA 16 0 O260200300044 ENDSUBENT 43 0 O260200399999 SUBENT O2602004 20240229 20260228 O260200400001 BIB 6 18 O260200400002 REACTION ((68-ER-168(P,2N)69-TM-167,,SIG,,FCT)+ O260200400003 (68-ER-167(P,N)69-TM-167,,SIG)) O260200400004 FCT=2.57/96.3 O260200400005 DECAY-DATA (69-TM-167,9.25D,DG,207.8,0.420) O260200400006 ERR-ANALYS (ERR-7) absolute gamma-ray intensity (19%) O260200400007 SAMPLE The enriched 167ErO3 sample with the following isotopicO260200400008 composition: O260200400009 Isotope: 162Er 164Er 166Er 167Er 168Er 170Er O260200400010 Abundance: <0.01 0.01 0.96 96.3 2.57 0.16 O260200400011 (68-ER-167,ENR=0.963) O260200400012 (68-ER-168,ENR=0.0257) O260200400013 COMMENT By compiler: Results reported as 167Er(p,x)167Tm O260200400014 compiled as sum of contributing reactions considering O260200400015 the reaction thresholds: O260200400016 167Tm production: Reaction; E threshold O260200400017 167Er+p; 1.5 MeV O260200400018 168Er+p; 9.4 MeV O260200400019 STATUS (TABLE,,E.Renaldin+,J,FRCH,2,1288588,2024) Table 3 O260200400020 ENDBIB 18 0 O260200400021 COMMON 1 3 O260200400022 ERR-7 O260200400023 PER-CENT O260200400024 19. O260200400025 ENDCOMMON 3 0 O260200400026 DATA 4 15 O260200400027 EN EN-ERR DATA ERR-T O260200400028 MEV MEV MB MB O260200400029 6.8 0.4 40.0 4.9 O260200400030 8.7 0.4 170. 34. O260200400031 9.7 0.4 303. 43. O260200400032 10.4 0.4 328. 47. O260200400033 11.1 0.4 399. 80. O260200400034 11.5 0.4 360. 73. O260200400035 12.1 0.4 290. 42. O260200400036 13.0 0.4 233. 48. O260200400037 14.1 0.4 149. 33. O260200400038 14.5 0.4 134. 17. O260200400039 15.2 0.4 119. 14. O260200400040 15.8 0.4 110. 13. O260200400041 16.5 0.4 105. 11. O260200400042 17.1 0.4 95.9 15.1 O260200400043 18.2 0.4 85.7 11.1 O260200400044 ENDDATA 17 0 O260200400045 ENDSUBENT 44 0 O260200499999 SUBENT O2602005 20240229 20260228 O260200500001 BIB 6 19 O260200500002 REACTION ((68-ER-170(P,3N)69-TM-168,,SIG,,FCT)+ O260200500003 (68-ER-168(P,N)69-TM-168,,SIG,,FCT)) O260200500004 FCT=0.16/96.3 for 170Er(p,3n) and 2.57/96.3 for O260200500005 168Er(p,n) O260200500006 DECAY-DATA (69-TM-168,93.1D,DG,198.3,0.545) O260200500007 SAMPLE The enriched 167ErO3 sample with the following isotopicO260200500008 composition: O260200500009 Isotope: 162Er 164Er 166Er 167Er 168Er 170Er O260200500010 Abundance: <0.01 0.01 0.96 96.3 2.57 0.16 O260200500011 (68-ER-168,ENR=0.0257) O260200500012 (68-ER-170,ENR=0.0016) O260200500013 COMMENT By compiler: Results reported as 167Er(p,x)168Tm O260200500014 compiled as sum of contributing reactions considering O260200500015 the reaction thresholds: O260200500016 168Tm production: Reaction; E threshold O260200500017 168Er+p; 2.5 MeV O260200500018 170Er+p; 15.8 MeV O260200500019 ERR-ANALYS (ERR-7) absolute gamma-ray intensity (5%) O260200500020 STATUS (TABLE,,E.Renaldin+,J,FRCH,2,1288588,2024) Table 3 O260200500021 ENDBIB 19 0 O260200500022 COMMON 1 3 O260200500023 ERR-7 O260200500024 PER-CENT O260200500025 5. O260200500026 ENDCOMMON 3 0 O260200500027 DATA 4 15 O260200500028 EN EN-ERR DATA ERR-T O260200500029 MEV MEV MB MB O260200500030 6.8 0.4 1.67 0.23 O260200500031 8.7 0.4 3.64 0.51 O260200500032 9.7 0.4 5.57 0.82 O260200500033 10.4 0.4 5.36 0.41 O260200500034 11.1 0.4 4.53 0.86 O260200500035 11.5 0.4 4.89 0.60 O260200500036 12.1 0.4 2.99 0.73 O260200500037 13.0 0.4 3.63 0.89 O260200500038 14.1 0.4 2.71 0.24 O260200500039 14.5 0.4 2.84 0.71 O260200500040 15.2 0.4 1.89 0.19 O260200500041 15.8 0.4 2.28 0.53 O260200500042 16.5 0.4 2.14 0.24 O260200500043 17.1 0.4 2.54 0.53 O260200500044 18.2 0.4 2.49 0.33 O260200500045 ENDDATA 17 0 O260200500046 ENDSUBENT 45 0 O260200599999 SUBENT O2602006 20240229 20260228 O260200600001 BIB 6 19 O260200600002 REACTION ((68-ER-167(P,3N)69-TM-165,,SIG,,FCT)+ O260200600003 (68-ER-166(P,2N)69-TM-165,,SIG,,FCT)) O260200600004 FCT=0.72/98.3 for 167Er(p,3n) and 0.37/98.3 for O260200600005 166Er(p,2n) O260200600006 DECAY-DATA (69-TM-165,30.06HR,DG,242.9,0.355) O260200600007 SAMPLE The enriched 168ErO3 sample with the following isotopicO260200600008 composition: O260200600009 Isotope: 166Er 167Er 168Er 170Er O260200600010 Abundance: 0.37 0.72 98.3 0.61 O260200600011 (68-ER-166,ENR=0.0037) O260200600012 (68-ER-167,ENR=0.0072) O260200600013 COMMENT By compiler: Results reported as 168Er(p,x)165Tm O260200600014 compiled as sum of contributing reactions considering O260200600015 the reaction thresholds: O260200600016 165Tm production: Reaction; E threshold O260200600017 166Er+p; 11.0 MeV O260200600018 167Er+p; 17.4 MeV O260200600019 ERR-ANALYS (ERR-7) absolute gamma-ray intensity (5%) O260200600020 STATUS (TABLE,,E.Renaldin+,J,FRCH,2,1288588,2024) Table 4 O260200600021 ENDBIB 19 0 O260200600022 COMMON 1 3 O260200600023 ERR-7 O260200600024 PER-CENT O260200600025 5. O260200600026 ENDCOMMON 3 0 O260200600027 DATA 4 6 O260200600028 EN EN-ERR DATA ERR-T O260200600029 MEV MEV MB MB O260200600030 13.0 0.4 1.62 0.18 O260200600031 14.1 0.4 1.53 0.15 O260200600032 15.2 0.4 2.73 1.01 O260200600033 16.4 0.4 3.34 0.37 O260200600034 17.1 0.4 3.21 0.40 O260200600035 18.2 0.4 3.31 0.41 O260200600036 ENDDATA 8 0 O260200600037 ENDSUBENT 36 0 O260200699999 SUBENT O2602007 20240229 20260228 O260200700001 BIB 6 19 O260200700002 REACTION ((68-ER-167(P,2N)69-TM-166,,SIG,,FCT)+ O260200700003 (68-ER-166(P,N)69-TM-166,,SIG,,FCT)) O260200700004 FCT=0.72/98.3 for 167Er(p,2n) and 0.37/98.3 for O260200700005 166Er(p,n) O260200700006 DECAY-DATA (69-TM-166-G,7.70HR,DG,778.8,0.191) O260200700007 SAMPLE The enriched 168ErO3 sample with the following isotopicO260200700008 composition: O260200700009 Isotope: 166Er 167Er 168Er 170Er O260200700010 Abundance: 0.37 0.72 98.3 0.61 O260200700011 (68-ER-166,ENR=0.0037) O260200700012 (68-ER-167,ENR=0.0072) O260200700013 COMMENT By compiler: Results reported as 168Er(p,x)166Tm O260200700014 compiled as sum of contributing reactions considering O260200700015 the reaction thresholds: O260200700016 166Tm production: Reaction; E threshold O260200700017 166Er+p; 3.8 MeV O260200700018 167Er+p; 10.3 MeV O260200700019 ERR-ANALYS (ERR-7) absolute gamma-ray intensity (5%) O260200700020 STATUS (TABLE,,E.Renaldin+,J,FRCH,2,1288588,2024) Table 4 O260200700021 ENDBIB 19 0 O260200700022 COMMON 1 3 O260200700023 ERR-7 O260200700024 PER-CENT O260200700025 5. O260200700026 ENDCOMMON 3 0 O260200700027 DATA 4 13 O260200700028 EN EN-ERR DATA ERR-T O260200700029 MEV MEV MB MB O260200700030 7.9 0.4 0.138 0.054 O260200700031 9.0 0.4 0.520 0.091 O260200700032 10.0 0.4 0.722 0.134 O260200700033 10.4 0.4 1.26 0.27 O260200700034 11.1 0.4 1.87 0.25 O260200700035 12.1 0.4 3.09 0.37 O260200700036 12.3 0.4 3.99 0.61 O260200700037 13.0 0.4 4.75 0.42 O260200700038 14.1 0.4 4.34 0.39 O260200700039 15.2 0.4 5.69 0.63 O260200700040 16.4 0.4 5.95 0.70 O260200700041 17.1 0.4 6.92 0.71 O260200700042 18.2 0.4 6.64 0.63 O260200700043 ENDDATA 15 0 O260200700044 ENDSUBENT 43 0 O260200799999 SUBENT O2602008 20240229 20260228 O260200800001 BIB 6 18 O260200800002 REACTION ((68-ER-168(P,2N)69-TM-167,,SIG)+ O260200800003 (68-ER-167(P,N)69-TM-167,,SIG,,FCT)) O260200800004 FCT=0.72/98.3 O260200800005 DECAY-DATA (69-TM-167,9.25D,DG,207.8,0.420) O260200800006 SAMPLE The enriched 168ErO3 sample with the following isotopicO260200800007 composition: O260200800008 Isotope: 166Er 167Er 168Er 170Er O260200800009 Abundance: 0.37 0.72 98.3 0.61 O260200800010 (68-ER-167,ENR=0.0072) O260200800011 (68-ER-168,ENR=0.983) O260200800012 COMMENT By compiler: Results reported as 168Er(p,x)167Tm O260200800013 compiled as sum of contributing reactions considering O260200800014 the reaction thresholds: O260200800015 167Tm production: Reaction; E threshold O260200800016 167Er+p; 1.5 MeV O260200800017 168Er+p; 9.4 MeV O260200800018 ERR-ANALYS (ERR-7) absolute gamma-ray intensity (19%) O260200800019 STATUS (TABLE,,E.Renaldin+,J,FRCH,2,1288588,2024) Table 4 O260200800020 ENDBIB 18 0 O260200800021 COMMON 1 3 O260200800022 ERR-7 O260200800023 PER-CENT O260200800024 19. O260200800025 ENDCOMMON 3 0 O260200800026 DATA 4 12 O260200800027 EN EN-ERR DATA ERR-T O260200800028 MEV MEV MB MB O260200800029 9.0 0.4 4.48 0.93 O260200800030 10.0 0.4 51.04 10.42 O260200800031 10.4 0.4 138. 28. O260200800032 11.1 0.4 279. 56. O260200800033 12.1 0.4 480. 97. O260200800034 12.3 0.4 533. 107. O260200800035 13.0 0.4 715. 144. O260200800036 14.1 0.4 675. 136. O260200800037 15.2 0.4 944. 190. O260200800038 16.4 0.4 888. 178. O260200800039 17.1 0.4 1112. 224. O260200800040 18.2 0.4 1178. 237. O260200800041 ENDDATA 14 0 O260200800042 ENDSUBENT 41 0 O260200899999 SUBENT O2602009 20240229 20260228 O260200900001 BIB 6 18 O260200900002 REACTION ((68-ER-170(P,3N)69-TM-168,,SIG,,FCT)+ O260200900003 (68-ER-168(P,N)69-TM-168,,SIG)) O260200900004 FCT=0.61/98.3 O260200900005 DECAY-DATA (69-TM-168,93.1D,DG,198.3,0.545) O260200900006 SAMPLE The enriched 168ErO3 sample with the following isotopicO260200900007 composition: O260200900008 Isotope: 166Er 167Er 168Er 170Er O260200900009 Abundance: 0.37 0.72 98.3 0.61 O260200900010 (68-ER-168,ENR=0.983) O260200900011 (68-ER-170,ENR=0.0061) O260200900012 COMMENT By compiler: Results reported as 168Er(p,x)168Tm O260200900013 compiled as sum of contributing reactions considering O260200900014 the reaction thresholds: O260200900015 168Tm production: Reaction; E threshold O260200900016 168Er+p; 2.5 MeV O260200900017 170Er+p; 15.8 MeV O260200900018 ERR-ANALYS (ERR-7) absolute gamma-ray intensity (5%) O260200900019 STATUS (TABLE,,E.Renaldin+,J,FRCH,2,1288588,2024) Table 4 O260200900020 ENDBIB 18 0 O260200900021 COMMON 1 3 O260200900022 ERR-7 O260200900023 PER-CENT O260200900024 5. O260200900025 ENDCOMMON 3 0 O260200900026 DATA 4 13 O260200900027 EN EN-ERR DATA ERR-T O260200900028 MEV MEV MB MB O260200900029 7.9 0.4 61.8 4.1 O260200900030 9.0 0.4 130. 9. O260200900031 10.0 0.4 198. 16. O260200900032 10.4 0.4 166. 33. O260200900033 11.1 0.4 137. 9. O260200900034 12.1 0.4 106. 7. O260200900035 12.3 0.4 99.7 7.1 O260200900036 13.0 0.4 86. 6.2 O260200900037 14.1 0.4 46. 4.3 O260200900038 15.2 0.4 46.4 3.6 O260200900039 16.4 0.4 48.3 5.4 O260200900040 17.1 0.4 41.8 2.7 O260200900041 18.2 0.4 36.2 4.6 O260200900042 ENDDATA 15 0 O260200900043 ENDSUBENT 42 0 O260200999999 ENDENTRY 9 0 O260299999999