ENTRY O1010 20191010 O072O101000000001 SUBENT O1010001 20191010 O072O101000100001 BIB 16 60 O101000100002 TITLE Measurements and nuclear model calculations on proton- O101000100003 induced reactions on Rh-103 up to 40-MeV-evaluation of O101000100004 the excitation function of the Rh-103(p,n)Pd-103 O101000100005 reaction relevant to the production of the therapeutic O101000100006 radionuclide Pd-103. O101000100007 AUTHOR (S.Sudar, F.Cserpak, S.M.Qaim) O101000100008 INSTITUTE (2GERJUL) O101000100009 (3HUNDEB) O101000100010 REFERENCE (J,ARI,56,821,2002) O101000100011 SAMPLE High-purity thin rhodium foils, O101000100012 isotopic composition- 99.9% Rh-103, thickness 25 mum, O101000100013 were used as samples. O101000100014 In a given stack about six such foils were placed. O101000100015 Copper monitor foils were inserted in each stack to O101000100016 degrade the proton energy as well as to determine the O101000100017 incident particle energy and the beam intensity. O101000100018 All the foils used were cut from materials of O101000100019 different thickness, thereby allowing changes in the O101000100020 mean energies of the irradiated rhodium samples. O101000100021 ADD-RES (COMP).Statistical model calculations. O101000100022 DETECTOR (LEGE) Low energy high purity Ge gamma detector O101000100023 (SILI) X-ray detector. O101000100024 ANALYSIS (AREA) O101000100025 (DECAY) O101000100026 MONITOR (29-CU-63(P,N)30-ZN-63,,SIG) O101000100027 (29-CU-65(P,N)30-ZN-65,,SIG) O101000100028 MONIT-REF (B0057001,R.COLLE+,J,PR/C,9,1819,1974) For Cu-63 O101000100029 target. O101000100030 (A0333001,P.KOPECKY,J,ARI,36,657,1985) For Cu-65 O101000100031 target. O101000100032 FACILITY (CYCLO,2GERJUL) At the compact cyclotron CV-28 and O101000100033 injector of COSY, Julich. O101000100034 The primary proton energies used were 15.8 and 19.6-MeVO101000100035 at the CV-28 and 45.1-MeV at the injector of COSY. O101000100036 CORRECTION *By authors*.The count rates were corrected for random O101000100037 pile-up losses as well as for gamma-ray abundance and O101000100038 the efficiency of the detector and self-absorption in O101000100039 the foils. Correction for coincidence loss was also O101000100040 taken into account. O101000100041 METHOD (STTA) See sample O101000100042 (BCINT) Besides monitor foils, the charge collected in O101000100043 a Faraday cup was also registered and there from the O101000100044 average beam current was deduced. The two results O101000100045 generally agreed within +/- 10%. O101000100046 (ACTIV) Each stack was irradiated for 30 - 60 minutes O101000100047 (EXTB) The primary proton energies used were 15.8 and O101000100048 19.6 MeV at the CV-28 and 45.1 MeV at the injector O101000100049 of COSY. O101000100050 (GSPEC) O101000100051 ERR-ANALYS (ERR-1).The error in beam intensity. O101000100052 (ERR-2).The error in detector efficiency. O101000100053 (ERR-3).Error in peak area and counting statistics. O101000100054 (ERR-4).Error in the number of target nuclei. O101000100055 (ERR-5).Error in the nuclear data. O101000100056 STATUS (TABLE).Data were taken from Table 2 of the original O101000100057 paper and from private communication. O101000100058 HISTORY (20021025C) O101000100059 (20080813A) Data were merged with D4125. O101000100060 (20090128A) Data were corrected O101000100061 (20191010A) SD: REACTION code corrected in Subent 005. O101000100062 ENDBIB 60 0 O101000100063 COMMON 5 3 O101000100064 ERR-1 ERR-2 ERR-3 ERR-4 ERR-5 O101000100065 PER-CENT PER-CENT PER-CENT PER-CENT PER-CENT O101000100066 7. 5. 25. 1.5 1. O101000100067 ENDCOMMON 3 0 O101000100068 ENDSUBENT 67 0 O101000199999 SUBENT O1010002 20090128 O039O101000200001 BIB 3 8 O101000200002 REACTION (45-RH-103(P,N)46-PD-103,,SIG) O101000200003 DECAY-DATA (46-PD-103,16.96D,XR,20.1/20.2,0.6502, O101000200004 DG,39.7,0.000683, O101000200005 DG,357.4,0.000221) O101000200006 ERR-ANALYS (EN-ERR).The uncertainty of the primary beam energy. O101000200007 The energy attenuation was calculated by using the O101000200008 method of Williamson. O101000200009 (ERR-T).Total error of the data. O101000200010 ENDBIB 8 0 O101000200011 NOCOMMON 0 0 O101000200012 DATA 4 26 O101000200013 EN EN-ERR DATA ERR-T O101000200014 MEV MEV MB MB O101000200015 2.99 0.25 2.2 0.13 O101000200016 5.31 0.25 61. 4. O101000200017 7.07 0.20 225. 12. O101000200018 8.62 0.20 445. 22. O101000200019 10.05 0.19 505. 26. O101000200020 11.34 0.19 383. 20. O101000200021 12.55 0.17 238. 12. O101000200022 13.53 0.17 162. 9. O101000200023 14.03 0.16 142. 8. O101000200024 14.46 0.16 114. 6. O101000200025 15.06 0.15 94. 5. O101000200026 15.35 0.15 82. 5. O101000200027 16.60 0.19 45. 3. O101000200028 17.52 0.18 36. 3. O101000200029 18.32 0.17 31. 3. O101000200030 18.4 0.16 28. 2. O101000200031 19.25 0.15 26. 2. O101000200032 21.54 0.28 24. 3. O101000200033 24.44 0.25 24. 3. O101000200034 26.46 0.23 25. 4. O101000200035 28.36 0.20 24. 5. O101000200036 30.75 0.19 24. 3. O101000200037 33.00 0.18 23. 4. O101000200038 35.15 0.17 21. 4. O101000200039 37.20 0.16 21. 4. O101000200040 39.65 0.15 16. 4. O101000200041 ENDDATA 28 0 O101000200042 ENDSUBENT 41 0 O101000299999 SUBENT O1010003 20090128 O039O101000300001 BIB 3 8 O101000300002 REACTION (45-RH-103(P,3N)46-PD-101,,SIG) O101000300003 DECAY-DATA (46-PD-101,8.46HR,DG,269.6,0.0643, O101000300004 DG,296.2,0.192, O101000300005 DG,590.4,0.1206) O101000300006 ERR-ANALYS (EN-ERR) The uncertainty of the primary beam energy. O101000300007 The energy attenuation was calculated by using the O101000300008 the method of Williamson. O101000300009 (ERR-T).Total error of the data. O101000300010 ENDBIB 8 0 O101000300011 NOCOMMON 0 0 O101000300012 DATA 4 9 O101000300013 EN EN-ERR DATA ERR-T O101000300014 MEV MEV MB MB O101000300015 21.54 0.28 91.1 8.0 O101000300016 24.44 0.25 360. 34. O101000300017 26.46 0.23 479. 41. O101000300018 28.36 0.20 547. 52. O101000300019 30.75 0.19 526. 47. O101000300020 33.00 0.18 531. 48. O101000300021 35.15 0.17 422. 36. O101000300022 37.20 0.16 333. 28. O101000300023 39.65 0.15 219. 22. O101000300024 ENDDATA 11 0 O101000300025 ENDSUBENT 24 0 O101000399999 SUBENT O1010004 20090128 O039O101000400001 BIB 3 7 O101000400002 REACTION (45-RH-103(P,4N)46-PD-100,,SIG) O101000400003 DECAY-DATA (46-PD-100,87.1HR,DG,74.8,0.441, O101000400004 DG,84.,0.45) O101000400005 ERR-ANALYS (EN-ERR) The uncertainty of the primary beam energy. O101000400006 The energy attenuation was calculated by using the O101000400007 method of Williamson. O101000400008 (ERR-T).Total error of the data. O101000400009 ENDBIB 7 0 O101000400010 NOCOMMON 0 0 O101000400011 DATA 4 5 O101000400012 EN EN-ERR DATA ERR-T O101000400013 MEV MEV MB MB O101000400014 30.75 0.19 5.1 0.9 O101000400015 33.00 0.18 49. 3. O101000400016 35.15 0.17 129. 10. O101000400017 37.20 0.16 218. 13. O101000400018 39.65 0.15 280. 19. O101000400019 ENDDATA 7 0 O101000400020 ENDSUBENT 19 0 O101000499999 SUBENT O1010005 20191010 O072O101000500001 BIB 4 21 O101000500002 REACTION 1(45-RH-103(P,N)46-PD-103,,SIG,,,EVAL) O101000500003 2(45-RH-103(P,N)46-PD-103,,TTY,,(PHY),EVAL) O101000500004 COMMENT *By authors*.The model calculated excitation function O101000500005 plays a transformation role for the data. We fitted theO101000500006 measured/model calculation ratio with a rational O101000500007 function, which described the deviation of the O101000500008 measured and calculated excitation function around O101000500009 20 MeV. For the fitting the 'TableCurve 2D' program O101000500010 of SPSS was used, taking into account in the weighting O101000500011 factor the uncertainties of the measurement. First we O101000500012 used all available data. Then we removed those series O101000500013 of measurements which had many data out of the 3 sigmaO101000500014 limit. In the next step all other data were fitted O101000500015 and again some points outside the 3s limit were O101000500016 removed. In the third step we got the final fit O101000500017 function (see fig.4). Table 3 gives the evaluated O101000500018 cross sections with the 95% confidence limits as well O101000500019 as the calculated integral yields of 103Pd. O101000500020 STATUS (TABLE) Table 3 from Appl.Rad.Isot.,56(2002)821 O101000500021 HISTORY (20191010A) SD: SF8=DT -> (PHY), SF9=DERIV -> EVAL in O101000500022 REACTION code (2). O101000500023 ENDBIB 21 0 O101000500024 NOCOMMON 0 0 O101000500025 DATA 3 74 O101000500026 EN DATA 1DATA 2 O101000500027 MEV MB MBQ/MUAHR O101000500028 3.0 0.28 O101000500029 3.5 1.4 O101000500030 4.0 5.0 O101000500031 4.5 14. 0.01 O101000500032 5.0 33. 0.03 O101000500033 5.5 65. 0.07 O101000500034 6.0 112. 0.15 O101000500035 6.5 171. 0.28 O101000500036 7.0 237. 0.50 O101000500037 7.5 305. 0.79 O101000500038 8.0 371. 1.2 O101000500039 8.5 431. 1.6 O101000500040 9.0 485. 2.2 O101000500041 9.5 500. 2.8 O101000500042 10.0 503. 3.5 O101000500043 10.5 459. 4.1 O101000500044 11.0 410. 4.7 O101000500045 11.5 353. 5.3 O101000500046 12.0 299. 5.8 O101000500047 12.5 249. 6.2 O101000500048 13.0 202. 6.5 O101000500049 13.5 166. 6.8 O101000500050 14.0 132. 7.1 O101000500051 14.5 109. 7.3 O101000500052 15.0 87. 7.5 O101000500053 15.5 72. 7.6 O101000500054 16.0 58. 7.7 O101000500055 16.5 50. 7.8 O101000500056 17.0 43. 7.9 O101000500057 17.5 36. 8.0 O101000500058 18.0 31. 8.1 O101000500059 18.5 28. 8.1 O101000500060 19.0 24. 8.2 O101000500061 19.5 23. 8.2 O101000500062 20.0 21. 8.3 O101000500063 20.5 20. 8.3 O101000500064 21.0 19. 8.4 O101000500065 21.5 18. 8.4 O101000500066 22.0 18. 8.5 O101000500067 22.5 19. 8.5 O101000500068 23.0 19. 8.5 O101000500069 23.5 19. 8.6 O101000500070 24.0 20. 8.6 O101000500071 24.5 20. 8.7 O101000500072 25.0 20. 8.7 O101000500073 25.5 21. 8.8 O101000500074 26.0 21. 8.8 O101000500075 26.5 22. 8.9 O101000500076 27.0 22. 9.0 O101000500077 27.5 22. 9.0 O101000500078 28.0 22. 9.1 O101000500079 28.5 22. 9.2 O101000500080 29.0 22. 9.2 O101000500081 29.5 23. 9.3 O101000500082 30.0 23. 9.3 O101000500083 30.5 23. 9.4 O101000500084 31.0 23. 9.5 O101000500085 31.5 22. 9.6 O101000500086 32.0 22. 9.6 O101000500087 32.5 22. 9.7 O101000500088 33.0 22. 9.8 O101000500089 33.5 22. 9.8 O101000500090 34.0 22. 9.9 O101000500091 34.5 22. 10.0 O101000500092 35.0 22. 10.0 O101000500093 35.5 22. 10.1 O101000500094 36.0 22. 10.2 O101000500095 36.5 21. 10.3 O101000500096 37.0 21. 10.3 O101000500097 37.5 21. 10.4 O101000500098 38.0 21. 10.5 O101000500099 38.5 21. 10.6 O101000500100 39.0 21. 10.6 O101000500101 39.5 21. 10.7 O101000500102 ENDDATA 76 0 O101000500103 ENDSUBENT 102 0 O101000599999 ENDENTRY 5 0 O101099999999