ENTRY O0845 20220111 O087O084500000001 SUBENT O0845001 20220111 O087O084500100001 BIB 16 64 O084500100002 TITLE Thin-target excitation functions, cross-sections and O084500100003 optimized thick-target yields for O084500100004 nat-Mo(p,xn)94g,95m,95g,96(m+g)Tc nuclear reactions O084500100005 induced by protons from threshold up to 44 MeV. No O084500100006 Carrier Added radiochemical separation and quality O084500100007 control O084500100008 AUTHOR (M.Bonardi, C.Birattari, F.Groppi, E.Sabbioni) O084500100009 REFERENCE (J,ARI,57,617,2002) O084500100010 REL-REF (M,B0038001,C.Birattari+,J,NP/A,166,605,1971) O084500100011 The "single target" activation technique at different O084500100012 proton energies. O084500100013 INSTITUTE (2ITYMIL) Radiochemistry laboratory. O084500100014 (2ZZZISP) Institute for health and consumer protection,O084500100015 SAMPLE High purity metallic Mo foils, the thickness uniformityO084500100016 determined was of 30.1 mu-m +/-1.4%, thus a 30.9 mg/cm2O084500100017 +/-1.4% mass thickness - measured by accurate O084500100018 weighting. O084500100019 MONITOR (6-C-12(P,X)6-C-11,,SIG) O084500100020 DETECTOR (GELI,HPGE) O084500100021 ANALYSIS (AREA) O084500100022 (DECAY) The decay of the different radionuclides has O084500100023 been followed for not less than three half-lives (1 O084500100024 year for the longer half-life radionuclides) and the O084500100025 times of measurement were chosen for each radionuclide O084500100026 so that the statistical error on the photo-peak area O084500100027 was always of the order of less than 0.1-1%. O084500100028 FACILITY (ISOCY,2ITYMIL) AVF cyclotron. O084500100029 The AVF cyclotron was a negative ions (H-) machine, O084500100030 with a thin Al stripping foil extraction system. O084500100031 METHOD (EXTB) A beam current of about 100 Na and an integratedO084500100032 charge varying from 200 to 400 mCoulomb. O084500100033 (BCINT) A long shaped Faraday cup. The beam intensity O084500100034 was checked by monitor reaction also, obtaining O084500100035 similar results within the 2%. O084500100036 (SITA,ACTIV,GSPEC) O084500100037 ERR-ANALYS (ERR-S,0.1,1.) The uncertainty of counting statistics O084500100038 (ERR-1) The uncertainty of target thickness O084500100039 (ERR-2) The uncertainty of efficiency calibration O084500100040 (ERR-3,1.,2.) The uncertainty of integrated charge O084500100041 (ERR-T) Overall error. The cumulative statistical O084500100042 errors on each thin-target yield data due to errors on O084500100043 photo-peak areas, decay constants, target thickness, O084500100044 integrated charge and detector efficiency, were O084500100045 smaller than a few percent. O084500100046 Systematic errors related to both stopping power O084500100047 calculations and absolute gamma-emission intensities O084500100048 were not considered. O084500100049 (EN-ERR) Includes energy losses in target and energy O084500100050 spread in beam. O084500100051 CORRECTION Cases requiring radioactive decay equilibrium O084500100052 considerations (A=95 and 96) were corrected using the O084500100053 equations of the radioactive chains. O084500100054 ADD-RES (TTY-C) O084500100055 Parameters of polynomials fittings and correlation O084500100056 factors for thin-target yields for the Tc radionuclidesO084500100057 STATUS (TABLE) Tbl.7,8 from Appl.Rad.Isot.,57(2002)617 O084500100058 HISTORY (20040204C) O084500100059 (20040212U) Last checking has been done. O084500100060 (20151203A) SD: DECAY-DATA corrected in Subent 005. O084500100061 SF5=IND (no mother nuclide) deleted from REACTION code;O084500100062 MISC -> DATA and second REACTION code was added in O084500100063 Subents 002-005. ERR-ANALYS update. O084500100064 (20170406A) SD: REACTION corrected in Subents 002,003. O084500100065 (20220111A) SD: Corrections in Subents 002,003. O084500100066 ENDBIB 64 0 O084500100067 COMMON 2 3 O084500100068 ERR-1 ERR-2 O084500100069 PER-CENT PER-CENT O084500100070 1.5 1.5 O084500100071 ENDCOMMON 3 0 O084500100072 ENDSUBENT 71 0 O084500199999 SUBENT O0845002 20220111 O087O084500200001 BIB 5 12 O084500200002 REACTION 1(42-MO-0(P,X)43-TC-94-G,,SIG) O084500200003 2(42-MO-0(P,X)43-TC-94-G,,TTY/DEN,,PHY) O084500200004 COMMENT - By compiler. Isomer transition <0.1%. O084500200005 DECAY-DATA (43-TC-94-G,4.883HR,DG,871.097,0.999, O084500200006 DG,702.639,0.996, O084500200007 DG,849.70,0.958) O084500200008 ADD-RES (DECAY) Half-life has been measured by authors O084500200009 T1/2=4.89 +/- 0.05 hours. O084500200010 HISTORY (20151204A) SD: second REACTION code was added; O084500200011 MISC -> DATA. O084500200012 (20220111A) SD: SF6=TTY -> TTY/DEN; SF8=TM -> PHY in O084500200013 REACTION (2) code. O084500200014 ENDBIB 12 0 O084500200015 NOCOMMON 0 0 O084500200016 DATA 6 17 O084500200017 EN EN-ERR DATA 1ERR-T 1DATA 2ERR-T 2O084500200018 MEV MEV MB MB MBQ/C/MEV MBQ/C/MEV O084500200019 4.9 1.5 4.2 0.15 174.9 6.3O084500200020 7.5 1.1 9.2 0.4 504.8 18.7O084500200021 9.9 0.8 13.6 0.5 908.7 30.9O084500200022 12.5 0.5 31.5 1. 2399.0 79.2O084500200023 15.1 0.3 57.8 1.9 4982.7 164.4O084500200024 17.4 0.2 66.7 2.2 6338.2 209.2O084500200025 20.0 0.2 72.8 2.4 7632.9 251.9O084500200026 22.6 0.2 76. 2.6 8707.1 296.0O084500200027 25.0 0.2 78.1 2.5 627.5 308.1O084500200028 27.5 0.2 80.8 2.7 10687.7 352.7O084500200029 30.0 0.2 79.5 2.6 11217.0 370.2O084500200030 32.5 0.2 79.6 2.6 11926.5 393.6O084500200031 34.4 0.2 79. 2.5 12344.9 395.0O084500200032 37.2 0.2 72.1 2.4 11955.2 394.5O084500200033 39.8 0.2 60.6 2. 10560.1 348.5O084500200034 41.6 0.2 58.4 2. 10521.3 357.7O084500200035 43.7 0.2 54.6 1.7 10208.7 326.7O084500200036 ENDDATA 19 0 O084500200037 ENDSUBENT 36 0 O084500299999 SUBENT O0845003 20220111 O087O084500300001 BIB 4 11 O084500300002 REACTION 1(42-MO-0(P,X)43-TC-95-M,,SIG) O084500300003 2(42-MO-0(P,X)43-TC-95-M,,TTY/DEN,,PHY) O084500300004 DECAY-DATA (43-TC-95-M,61.D,DG,204.114,0.662, O084500300005 DG,582.062,0.314, O084500300006 DG,835.126,0.279) O084500300007 ADD-RES (DECAY) Half-life has been measured by authors. O084500300008 T1/2=61.3 +/- 0.5 days. O084500300009 HISTORY (20151204A) SD: second REACTION code was added; O084500300010 MISC -> DATA. O084500300011 (20220111A) SD: SF6=TTY -> TTY/DEN; SF8=TM -> PHY in O084500300012 REACTION (2) code. O084500300013 ENDBIB 11 0 O084500300014 NOCOMMON 0 0 O084500300015 DATA 6 17 O084500300016 EN EN-ERR DATA 1ERR-T 1DATA 2ERR-T 2O084500300017 MEV MEV MB MB MBQ/C/MEV MBQ/C/MEV O084500300018 4.9 1.5 20.6 0.7 2.84 0.09O084500300019 7.5 1.1 29.7 1.0 5.44 0.19O084500300020 9.9 0.8 34.3 1.1 7.62 0.25O084500300021 12.5 0.5 47.5 1.5 12.08 0.39O084500300022 15.1 0.3 54.7 1.8 15.72 0.52O084500300023 17.4 0.2 52.7 1.7 16.71 0.55O084500300024 20.0 0.2 48.6 1.6 16.97 0.58O084500300025 22.6 0.2 50.2 1.6 19.15 0.61O084500300026 25.0 0.2 41.9 1.4 17.20 0.57O084500300027 27.5 0.2 33.3 1.1 14.67 0.50O084500300028 30.0 0.2 27.7 0.9 13.01 0.42O084500300029 32.5 0.2 27.3 0.9 13.61 0.46O084500300030 34.4 0.2 30.0 1.0 15.62 0.53O084500300031 37.2 0.2 32.0 1.1 17.66 0.58O084500300032 39.8 0.2 30.8 1.0 17.88 0.57O084500300033 41.6 0.2 30.0 1.0 18.00 0.59O084500300034 43.7 0.2 28.4 0.9 17.72 0.58O084500300035 ENDDATA 19 0 O084500300036 ENDSUBENT 35 0 O084500399999 SUBENT O0845004 20170406 O061O084500400001 BIB 5 11 O084500400002 REACTION 1(42-MO-0(P,X)43-TC-95-G,M+,SIG) O084500400003 2(42-MO-0(P,X)43-TC-95-G,M+,TTY/DEN,,PHY) O084500400004 COMMENT - By authors. Isomer transition 4%. O084500400005 DECAY-DATA (43-TC-95-G,20.HR,DG,765.789,0.940, O084500400006 DG,1073.713,0.037) O084500400007 ADD-RES (DECAY) Half-life has been measured by authors. O084500400008 T1/2=19.7 +/- 0.7 hours. O084500400009 HISTORY (20151204A) SD: SF5=M+ (IT=4%) added to REACTION code. O084500400010 Second REACTION code was added; MISC -> DATA. O084500400011 (20170402A) SD: SF6=TTY -> TTY/DEN, SF8=TM -> PHY in O084500400012 REACTION (2) code. O084500400013 ENDBIB 11 0 O084500400014 NOCOMMON 0 0 O084500400015 DATA 6 17 O084500400016 EN EN-ERR DATA 1ERR-T 1DATA 2ERR-T 2O084500400017 MEV MEV MB MB MBQ/C/MEV MBQ/C/MEV O084500400018 4.9 1.5 50.3 2.1 506.8 21.3O084500400019 7.5 1.1 70.9 2.9 951.8 39.O084500400020 9.9 0.8 80.8 3.4 1312.2 55.1O084500400021 12.5 0.5 118.2 4.8 2200.1 90.2O084500400022 15.1 0.3 127.3 5.2 2678.7 109.8O084500400023 17.4 0.2 125.6 5.1 2913.8 119.5O084500400024 20. 0.2 136.9 5.7 3501.7 147.1O084500400025 22.6 0.2 160.3 6.6 4478.1 183.6O084500400026 25. 0.2 144.3 6.2 4340.8 186.6O084500400027 27.5 0.2 120.5 4.9 3888.6 159.4O084500400028 30. 0.2 104.6 4.7 3601.2 162.O084500400029 32.5 0.2 110.3 4.7 4030.7 173.3O084500400030 34.4 0.2 119.7 5.1 4564.4 196.3O084500400031 37.2 0.2 117.1 5.3 4735.6 213.1O084500400032 39.8 0.2 121.1 5. 5149.5 211.1O084500400033 41.6 0.2 131.2 5.5 5767.1 242.2O084500400034 43.7 0.2 122.9 5.4 5607. 246.7O084500400035 ENDDATA 19 0 O084500400036 ENDSUBENT 35 0 O084500499999 SUBENT O0845005 20170406 O061O084500500001 BIB 5 12 O084500500002 REACTION 1(42-MO-0(P,X)43-TC-96-G,M+,SIG) O084500500003 2(42-MO-0(P,X)43-TC-96-G,M+,TTY/DEN,,PHY) O084500500004 COMMENT - By compiler. Isomer transition 98%. O084500500005 DECAY-DATA (43-TC-96-G,4.28D,DG,778.196,0.9978, O084500500006 DG,849.89,0.98, O084500500007 DG,812.54,0.82) O084500500008 ADD-RES (DECAY) Half-life has been measured by authors. O084500500009 T1/2=4.24 +/- 0.08 days. O084500500010 HISTORY (20151203A) SD: Tc-95g -> TC-96g in DECAY-DATA. O084500500011 Second REACTION code was added; MISC -> DATA. O084500500012 (20170402A) SD: SF6=TTY -> TTY/DEN, SF8=TM -> PHY in O084500500013 REACTION (2) code. O084500500014 ENDBIB 12 0 O084500500015 NOCOMMON 0 0 O084500500016 DATA 6 17 O084500500017 EN EN-ERR DATA 1ERR-T 1DATA 2ERR-T 2O084500500018 MEV MEV MB MB MBQ/C/MEV MBQ/C/MEV O084500500019 4.9 1.5 74.6 2.5 146.4 5.O084500500020 7.5 1.1 108.4 3.7 283.5 9.6O084500500021 9.9 0.8 142.1 4.8 449.5 15.3O084500500022 12.5 0.5 154.4 5.2 559.4 19.O084500500023 15.1 0.3 126.3 4.3 517.4 17.6O084500500024 17.4 0.2 118.2 4. 534. 18.1O084500500025 20. 0.2 113.2 3.8 563.8 19.2O084500500026 22.6 0.2 149.5 4.9 813.4 26.8O084500500027 25. 0.2 199.8 6.6 1170. 38.6O084500500028 27.5 0.2 222.2 7.6 1395.9 47.5O084500500029 30. 0.2 224.7 7.2 1505.8 48.2O084500500030 32.5 0.2 214.1 7.1 1523.8 50.3O084500500031 34.4 0.2 173.8 6.3 1289.8 46.4O084500500032 37.2 0.2 122. 4. 960.2 31.7O084500500033 39.8 0.2 92. 3.1 761.7 25.9O084500500034 41.6 0.2 82.4 2.7 705.5 23.3O084500500035 43.7 0.2 83.1 2.8 738.1 25.1O084500500036 ENDDATA 19 0 O084500500037 ENDSUBENT 36 0 O084500599999 ENDENTRY 5 0 O084599999999