ENTRY D4411 20210105 D130D441100000001 SUBENT D4411001 20210105 D130D441100100001 BIB 13 44 D441100100002 TITLE Investigation of the deuteron induced nuclear reaction D441100100003 cross sections on lutetium up to 50 MeV: review of D441100100004 production routes for 177Lu, 175Hf and 172Hf via D441100100005 charged particle activation D441100100006 AUTHOR (F.Tarkanyi,S.Takacs,F.Ditroi,A.Hermanne, D441100100007 R.Adam-Rebeles,A.V.Ignatyuk) D441100100008 INSTITUTE (3HUNDEB,2BLGVUB,4RUSFEI) D441100100009 REFERENCE (J,JRN,324,1405,2020) D441100100010 #doi:10.1007/s10967-020-07182-w D441100100011 SAMPLE High purity natural lutetium foils 110 um from D441100100012 Goodfellow. D441100100013 Al 27 um monitor foils. D441100100014 DETECTOR (HPGE) D441100100015 FACILITY (CYCLO,2BLGLVN) D441100100016 METHOD (STTA,ACTIV,EXTB,GSPEC) D441100100017 One stack consisted of 25 Lu target foils D441100100018 and Al foils for beam monitoring was bombarded for D441100100019 40 min with a 50 MeV deuteron beam of 110 nA. D441100100020 MONITOR (13-AL-27(D,X)11-NA-24,,SIG) D441100100021 (13-AL-27(D,X)11-NA-22,,SIG) D441100100022 MONIT-REF (,,R,IAEA-NDS-1211,2001) D441100100023 ERR-ANALYS (EN-ERR)The uncertainty of the beam energy in the D441100100024 middle of each irradiated foil was estimated D441100100025 combining the uncertainties of the energy degradation D441100100026 depending on the thickness of the target foils in the D441100100027 stack and the energy straggling (+-0.3 to 1.1 MeV) D441100100028 (ERR-T)The uncertainty on the cross-section was D441100100029 estimated by taking the square root of the sum in D441100100030 quadrature of all individual contributions, supposing D441100100031 equal sensitivities for the different parameters. D441100100032 The main error components: D441100100033 (ERR-1)surface density of target nuclei (5 %) D441100100034 (ERR-2)incident charged particle flux (7 %) D441100100035 (ERR-3,5.,7.)detector efficiency (5-7 %) D441100100036 (ERR-4,1.,3.)gamma intensities (1-3 %) D441100100037 (ERR-S,1.,18.) statistical uncertainty (1.0-18. %) D441100100038 ADD-RES (THEO) The experimental data were compared to the D441100100039 results of the theoretical model calculations by D441100100040 ALICE-IPPE-D, EMPIRE-D TALYS 1.9 codes. D441100100041 (TTY-C) Fitted excitation functions were used for D441100100042 determination of integral physical yields. D441100100043 (COMP) The measured experimental data were compared to D441100100044 those found in the literature. D441100100045 HISTORY (20210105C) ts D441100100046 ENDBIB 44 0 D441100100047 COMMON 2 3 D441100100048 ERR-1 ERR-2 D441100100049 PER-CENT PER-CENT D441100100050 5. 7. D441100100051 ENDCOMMON 3 0 D441100100052 ENDSUBENT 51 0 D441100199999 SUBENT D4411002 20210105 D130D441100200001 BIB 3 5 D441100200002 REACTION (71-LU-0(D,X)72-HF-175,,SIG) D441100200003 DECAY-DATA (72-HF-175,70.D,DG,343.40,0.840) D441100200004 STATUS (TABLE) Decay data are from table2, cross section data D441100200005 are from table3 of D441100200006 J. Radioanal. Nucl. Chem.,324,1405,2020 D441100200007 ENDBIB 5 0 D441100200008 NOCOMMON 0 0 D441100200009 DATA 4 24 D441100200010 EN EN-ERR DATA ERR-T D441100200011 MEV MEV MB MB D441100200012 49.4 0.3 44.1 5.4 D441100200013 48.2 0.3 46.1 5.6 D441100200014 46.9 0.3 48.6 5.9 D441100200015 45.6 0.4 49.3 6.0 D441100200016 44.3 0.4 51.7 6.2 D441100200017 43.0 0.4 55.5 6.7 D441100200018 41.6 0.4 58.3 7.0 D441100200019 40.2 0.5 60.6 7.3 D441100200020 38.7 0.5 62.8 7.6 D441100200021 37.2 0.5 70.9 8.5 D441100200022 35.7 0.5 74.9 9.0 D441100200023 34.1 0.6 81.1 9.7 D441100200024 32.5 0.6 85.8 10.3 D441100200025 30.8 0.6 91.3 10.9 D441100200026 29.0 0.7 103.5 12.4 D441100200027 27.2 0.7 114.5 13.7 D441100200028 25.3 0.8 137.3 16.4 D441100200029 23.2 0.8 161.1 19.2 D441100200030 21.1 0.9 202.0 24.1 D441100200031 18.7 0.9 291.2 34.7 D441100200032 16.2 1.0 450.4 53.7 D441100200033 13.4 1.0 499.4 59.5 D441100200034 10.0 1.1 150.1 17.9 D441100200035 5.7 1.2 2.6 0.3 D441100200036 ENDDATA 26 0 D441100200037 ENDSUBENT 36 0 D441100299999 SUBENT D4411003 20210105 D130D441100300001 BIB 3 5 D441100300002 REACTION (71-LU-0(D,X)72-HF-173,,SIG) D441100300003 DECAY-DATA (72-HF-173,23.6HR,DG,123.675,0.83) D441100300004 STATUS (TABLE) Decay data are from table2, cross section data D441100300005 are from table3 of D441100300006 J. Radioanal. Nucl. Chem.,324,1405,2020 D441100300007 ENDBIB 5 0 D441100300008 NOCOMMON 0 0 D441100300009 DATA 4 20 D441100300010 EN EN-ERR DATA ERR-T D441100300011 MEV MEV MB MB D441100300012 49.4 0.3 306.5 36.6 D441100300013 48.2 0.3 330.0 39.4 D441100300014 46.9 0.3 354.0 42.2 D441100300015 45.6 0.4 375.4 44.8 D441100300016 44.3 0.4 403.8 48.2 D441100300017 43.0 0.4 453.5 54.1 D441100300018 41.6 0.4 503.1 60.0 D441100300019 40.2 0.5 559.4 66.7 D441100300020 38.7 0.5 624.3 74.4 D441100300021 37.2 0.5 762.8 90.9 D441100300022 35.7 0.5 843.3 100.5 D441100300023 34.1 0.6 923.9 110.1 D441100300024 32.5 0.6 978.1 116.6 D441100300025 30.8 0.6 927.5 110.6 D441100300026 29.0 0.7 809.1 96.5 D441100300027 27.2 0.7 585.5 69.8 D441100300028 25.3 0.8 345.4 41.2 D441100300029 23.2 0.8 97.6 11.7 D441100300030 21.1 0.9 6.5 0.8 D441100300031 18.7 0.9 0.3 0.1 D441100300032 ENDDATA 22 0 D441100300033 ENDSUBENT 32 0 D441100399999 SUBENT D4411004 20210105 D130D441100400001 BIB 3 5 D441100400002 REACTION (71-LU-0(D,X)72-HF-172,,SIG) D441100400003 DECAY-DATA (72-HF-172,1.87YR,DG,125.812,0.113) D441100400004 STATUS (TABLE) Decay data are from table2, cross section data D441100400005 are from table3 of D441100400006 J. Radioanal. Nucl. Chem.,324,1405,2020 D441100400007 ENDBIB 5 0 D441100400008 NOCOMMON 0 0 D441100400009 DATA 4 14 D441100400010 EN EN-ERR DATA ERR-T D441100400011 MEV MEV MB MB D441100400012 49.4 0.3 531.2 63.6 D441100400013 48.2 0.3 567.1 68.2 D441100400014 46.9 0.3 641.4 76.8 D441100400015 45.6 0.4 649.0 77.7 D441100400016 44.3 0.4 686.6 82.2 D441100400017 43.0 0.4 706.5 85.1 D441100400018 41.6 0.4 696.7 85.0 D441100400019 40.2 0.5 596.4 71.3 D441100400020 38.7 0.5 505.5 62.2 D441100400021 37.2 0.5 428.6 55.3 D441100400022 35.7 0.5 266.8 34.9 D441100400023 34.1 0.6 150.4 19.9 D441100400024 32.5 0.6 60.2 11.4 D441100400025 30.8 0.6 4.2 2.2 D441100400026 ENDDATA 16 0 D441100400027 ENDSUBENT 26 0 D441100499999 SUBENT D4411005 20210105 D130D441100500001 BIB 3 6 D441100500002 REACTION (71-LU-0(D,X)72-HF-171,,SIG) D441100500003 DECAY-DATA (72-HF-171-G,12.1HR,DG,347.20,0.06) Relative gamma D441100500004 intensity (150) was multiplied by the factor of 0.04. D441100500005 STATUS (TABLE) Decay data are from table2, cross section data D441100500006 are from table3 of D441100500007 J. Radioanal. Nucl. Chem.,324,1405,2020 D441100500008 ENDBIB 6 0 D441100500009 NOCOMMON 0 0 D441100500010 DATA 4 8 D441100500011 EN EN-ERR DATA ERR-T D441100500012 MEV MEV MB MB D441100500013 49.4 0.3 388.7 46.5 D441100500014 48.2 0.3 310.4 37.1 D441100500015 46.9 0.3 231.5 27.7 D441100500016 45.6 0.4 149.9 18.0 D441100500017 44.3 0.4 87.6 10.6 D441100500018 43.0 0.4 40.0 4.9 D441100500019 41.6 0.4 13.8 1.9 D441100500020 40.2 0.5 2.7 0.6 D441100500021 ENDDATA 10 0 D441100500022 ENDSUBENT 21 0 D441100599999 SUBENT D4411006 20210105 D130D441100600001 BIB 3 5 D441100600002 REACTION (71-LU-0(D,X)71-LU-177-M,,SIG) D441100600003 DECAY-DATA (71-LU-177-M,160.44D,DG,418.54,0.2172) D441100600004 STATUS (TABLE) Decay data are from table2, cross section data D441100600005 are from table5 of D441100600006 J. Radioanal. Nucl. Chem.,324,1405,2020 D441100600007 ENDBIB 5 0 D441100600008 NOCOMMON 0 0 D441100600009 DATA 4 6 D441100600010 EN EN-ERR DATA ERR-T D441100600011 MEV MEV MB MB D441100600012 29.0 0.7 0.38 0.15 D441100600013 25.3 0.8 0.32 0.12 D441100600014 18.7 0.9 1.16 0.37 D441100600015 13.4 1.0 1.32 0.30 D441100600016 10.0 1.1 0.91 0.24 D441100600017 5.7 1.2 0.60 0.17 D441100600018 ENDDATA 8 0 D441100600019 ENDSUBENT 18 0 D441100699999 SUBENT D4411007 20210105 D130D441100700001 BIB 4 7 D441100700002 REACTION (71-LU-0(D,X)71-LU-177-G,,SIG) D441100700003 DECAY-DATA (71-LU-177-G,6.647D,DG,208.3662,0.1041) D441100700004 CORRECTION Not corrected for contribution from decay of 177mLu, D441100700005 which fraction was negligible small. D441100700006 STATUS (TABLE) Decay data are from table2, cross section data D441100700007 are from table5 of D441100700008 J. Radioanal. Nucl. Chem.,324,1405,2020 D441100700009 ENDBIB 7 0 D441100700010 NOCOMMON 0 0 D441100700011 DATA 4 19 D441100700012 EN EN-ERR DATA ERR-T D441100700013 MEV MEV MB MB D441100700014 49.4 0.3 1.86 0.31 D441100700015 48.2 0.3 2.26 0.34 D441100700016 46.9 0.3 2.25 0.35 D441100700017 45.6 0.4 2.37 0.34 D441100700018 44.3 0.4 2.81 0.37 D441100700019 43.0 0.4 2.60 0.34 D441100700020 41.6 0.4 2.77 0.79 D441100700021 40.2 0.5 2.86 0.74 D441100700022 38.7 0.5 2.09 0.27 D441100700023 37.2 0.5 3.20 0.69 D441100700024 35.7 0.5 2.25 0.31 D441100700025 34.1 0.6 2.75 0.36 D441100700026 32.5 0.6 3.26 0.43 D441100700027 30.8 0.6 3.50 0.45 D441100700028 29.0 0.7 5.26 1.13 D441100700029 27.2 0.7 4.86 1.02 D441100700030 25.3 0.8 2.91 0.35 D441100700031 23.2 0.8 0.35 0.05 D441100700032 21.1 0.9 0.25 0.08 D441100700033 ENDDATA 21 0 D441100700034 ENDSUBENT 33 0 D441100799999 SUBENT D4411008 20210105 D130D441100800001 BIB 3 5 D441100800002 REACTION (71-LU-0(D,X)71-LU-176-M,,SIG) D441100800003 DECAY-DATA (71-LU-176-M,3.635HR,DG,88.361,0.089) D441100800004 STATUS (TABLE) Decay data are from table2, cross section data D441100800005 are from table5 of D441100800006 J. Radioanal. Nucl. Chem.,324,1405,2020 D441100800007 ENDBIB 5 0 D441100800008 NOCOMMON 0 0 D441100800009 DATA 4 24 D441100800010 EN EN-ERR DATA ERR-T D441100800011 MEV MEV MB MB D441100800012 49.4 0.3 32.0 4.5 D441100800013 48.2 0.3 17.1 3.4 D441100800014 46.9 0.3 31.7 4.2 D441100800015 45.6 0.4 23.5 3.3 D441100800016 44.3 0.4 22.0 2.9 D441100800017 43.0 0.4 20.7 2.8 D441100800018 41.6 0.4 22.3 3.2 D441100800019 40.2 0.5 41.4 5.1 D441100800020 38.7 0.5 41.6 5.2 D441100800021 37.2 0.5 42.5 5.2 D441100800022 35.7 0.5 46.6 5.8 D441100800023 34.1 0.6 51.6 6.3 D441100800024 32.5 0.6 55.1 6.7 D441100800025 30.8 0.6 20.1 2.8 D441100800026 29.0 0.7 41.0 5.1 D441100800027 27.2 0.7 37.6 4.6 D441100800028 25.3 0.8 48.5 5.9 D441100800029 23.2 0.8 50.1 6.0 D441100800030 21.1 0.9 58.5 7.0 D441100800031 18.7 0.9 69.6 8.3 D441100800032 16.2 1.0 86.1 10.3 D441100800033 13.4 1.0 100.2 12.0 D441100800034 10.0 1.1 52.8 6.4 D441100800035 5.7 1.2 5.4 0.7 D441100800036 ENDDATA 26 0 D441100800037 ENDSUBENT 36 0 D441100899999 SUBENT D4411009 20210105 D130D441100900001 BIB 4 7 D441100900002 REACTION (71-LU-0(D,X)71-LU-174-G,,SIG) D441100900003 DECAY-DATA (71-LU-174-G,3.31YR,DG,1241.847,0.0514) D441100900004 STATUS (TABLE) Decay data are from table2, cross section data D441100900005 are from table4 of D441100900006 J. Radioanal. Nucl. Chem.,324,1405,2020 D441100900007 CORRECTION Isomeric transition contribution subtracted by using D441100900008 174mLu production cross section predicted by TENDL2019.D441100900009 ENDBIB 7 0 D441100900010 NOCOMMON 0 0 D441100900011 DATA 4 18 D441100900012 EN EN-ERR DATA ERR-T D441100900013 MEV MEV MB MB D441100900014 49.4 0.3 73.8 1.6 D441100900015 46.9 0.3 159.0 2.2 D441100900016 45.6 0.4 100.3 0.0 D441100900017 44.3 0.4 130.2 1.3 D441100900018 43.0 0.4 188.1 1.7 D441100900019 41.6 0.4 164.0 1.9 D441100900020 40.2 0.5 147.1 2.3 D441100900021 38.7 0.5 135.3 2.2 D441100900022 37.2 0.5 175.9 2.4 D441100900023 35.7 0.5 157.8 2.8 D441100900024 34.1 0.6 154.4 2.6 D441100900025 32.5 0.6 159.2 2.8 D441100900026 30.8 0.6 114.4 2.9 D441100900027 29.0 0.7 83.4 2.1 D441100900028 27.2 0.7 90.7 3.2 D441100900029 25.3 0.8 51.6 2.2 D441100900030 23.2 0.8 31.0 2.8 D441100900031 21.1 0.9 35.5 3.3 D441100900032 ENDDATA 20 0 D441100900033 ENDSUBENT 32 0 D441100999999 SUBENT D4411010 20210105 D130D441101000001 BIB 4 7 D441101000002 REACTION (71-LU-0(D,X)71-LU-173,,SIG) D441101000003 DECAY-DATA (71-LU-173,1.37YR,DG,272.105,0.212) D441101000004 STATUS (TABLE) Decay data are from table2, cross section data D441101000005 are from table4 of D441101000006 J. Radioanal. Nucl. Chem.,324,1405,2020 D441101000007 CORRECTION 173Hf decay contribution subtracted by using the D441101000008 measured 173Hf production cross section. D441101000009 ENDBIB 7 0 D441101000010 NOCOMMON 0 0 D441101000011 DATA 4 15 D441101000012 EN EN-ERR DATA ERR-T D441101000013 MEV MEV MB MB D441101000014 49.4 0.3 212.6 53.2 D441101000015 48.2 0.3 219.4 56.8 D441101000016 46.9 0.3 192.2 58.3 D441101000017 45.6 0.4 193.0 61.1 D441101000018 44.3 0.4 182.8 64.5 D441101000019 43.0 0.4 164.8 70.7 D441101000020 41.6 0.4 143.3 77.0 D441101000021 40.2 0.5 128.4 84.7 D441101000022 38.7 0.5 118.9 93.9 D441101000023 37.2 0.5 128.4 114.4 D441101000024 35.7 0.5 97.1 125.7 D441101000025 34.1 0.6 76.6 137.3 D441101000026 32.5 0.6 58.4 145.1 D441101000027 30.8 0.6 31.3 137.4 D441101000028 29.0 0.7 16.4 119.8 D441101000029 ENDDATA 17 0 D441101000030 ENDSUBENT 29 0 D441101099999 SUBENT D4411011 20210105 D130D441101100001 BIB 3 5 D441101100002 REACTION (71-LU-0(D,X)71-LU-173,CUM,SIG) D441101100003 DECAY-DATA (71-LU-173,1.37YR,DG,272.105,0.212) D441101100004 STATUS (TABLE) Decay data are from table2, cross section data D441101100005 are from table4 of D441101100006 J. Radioanal. Nucl. Chem.,324,1405,2020 D441101100007 ENDBIB 5 0 D441101100008 NOCOMMON 0 0 D441101100009 DATA 4 20 D441101100010 EN EN-ERR DATA ERR-T D441101100011 MEV MEV MB MB D441101100012 49.4 0.3 531.0 65.4 D441101100013 48.2 0.3 562.3 67.2 D441101100014 46.9 0.3 556.6 70.8 D441101100015 45.6 0.4 577.7 70.6 D441101100016 44.3 0.4 595.6 71.1 D441101100017 43.0 0.4 627.0 75.2 D441101100018 41.6 0.4 654.2 78.1 D441101100019 40.2 0.5 695.0 83.8 D441101100020 38.7 0.5 750.3 90.1 D441101100021 37.2 0.5 899.6 107.8 D441101100022 35.7 0.5 948.7 113.5 D441101100023 34.1 0.6 1008.7 120.4 D441101100024 32.5 0.6 1044.3 124.8 D441101100025 30.8 0.6 965.7 115.4 D441101100026 29.0 0.7 831.4 99.4 D441101100027 27.2 0.7 585.6 70.1 D441101100028 25.3 0.8 342.5 40.9 D441101100029 23.2 0.8 97.3 11.7 D441101100030 21.1 0.9 11.4 1.7 D441101100031 18.7 0.9 2. 1. D441101100032 ENDDATA 22 0 D441101100033 ENDSUBENT 32 0 D441101199999 SUBENT D4411012 20210105 D130D441101200001 BIB 3 5 D441101200002 REACTION (71-LU-0(D,X)71-LU-172,,SIG) D441101200003 DECAY-DATA (71-LU-172-G,6.70D,DG,181.525,0.206) D441101200004 STATUS (TABLE) Decay data are from table2, cross section data D441101200005 are from table4 of D441101200006 J. Radioanal. Nucl. Chem.,324,1405,2020 D441101200007 ENDBIB 5 0 D441101200008 NOCOMMON 0 0 D441101200009 DATA 4 19 D441101200010 EN EN-ERR DATA ERR-T D441101200011 MEV MEV MB MB D441101200012 49.4 0.3 81.4 9.8 D441101200013 48.2 0.3 72.6 8.8 D441101200014 46.9 0.3 61.8 7.4 D441101200015 45.6 0.4 54.0 6.6 D441101200016 44.3 0.4 43.0 5.3 D441101200017 43.0 0.4 34.1 4.1 D441101200018 41.6 0.4 25.6 3.3 D441101200019 40.2 0.5 19.2 2.6 D441101200020 38.7 0.5 13.6 2.0 D441101200021 37.2 0.5 9.2 1.2 D441101200022 35.7 0.5 6.1 1.0 D441101200023 34.1 0.6 4.5 0.6 D441101200024 32.5 0.6 2.7 0.4 D441101200025 30.8 0.6 2.6 0.9 D441101200026 29.0 0.7 0.7 0.1 D441101200027 27.2 0.7 0.7 0.2 D441101200028 25.3 0.8 0.5 0.2 D441101200029 23.2 0.8 0.5 0.1 D441101200030 21.1 0.9 0.3 0.2 D441101200031 ENDDATA 21 0 D441101200032 ENDSUBENT 31 0 D441101299999 SUBENT D4411013 20210105 D130D441101300001 BIB 3 5 D441101300002 REACTION (71-LU-0(D,X)71-LU-171,CUM,SIG) D441101300003 DECAY-DATA (71-LU-171-G,8.24D,DG,739.793,0.487) D441101300004 STATUS (TABLE) Decay data are from table2, cross section data D441101300005 are from table4 of D441101300006 J. Radioanal. Nucl. Chem.,324,1405,2020 D441101300007 ENDBIB 5 0 D441101300008 NOCOMMON 0 0 D441101300009 DATA 4 11 D441101300010 EN EN-ERR DATA ERR-T D441101300011 MEV MEV MB MB D441101300012 49.4 0.3 372. 44. D441101300013 48.2 0.3 296. 35. D441101300014 46.9 0.3 216. 26. D441101300015 45.6 0.4 144. 17. D441101300016 44.3 0.4 84. 10. D441101300017 43.0 0.4 40. 5. D441101300018 41.6 0.4 15. 2. D441101300019 40.2 0.5 4.7 0.6 D441101300020 38.7 0.5 1.2 0.2 D441101300021 37.2 0.5 0.14 0.08 D441101300022 35.7 0.5 0.22 0.08 D441101300023 ENDDATA 13 0 D441101300024 ENDSUBENT 23 0 D441101399999 SUBENT D4411014 20210105 D130D441101400001 BIB 3 5 D441101400002 REACTION (71-LU-0(D,X)70-YB-169,,SIG) D441101400003 DECAY-DATA (70-YB-169-G,32.018D,DG,197.95675,0.3593) D441101400004 STATUS (TABLE) Decay data are from table2, cross section data D441101400005 are from table5 of D441101400006 J. Radioanal. Nucl. Chem.,324,1405,2020 D441101400007 ENDBIB 5 0 D441101400008 NOCOMMON 0 0 D441101400009 DATA 4 10 D441101400010 EN EN-ERR DATA ERR-T D441101400011 MEV MEV MB MB D441101400012 49.4 0.3 15.9 1.9 D441101400013 48.2 0.3 15.2 1.8 D441101400014 46.9 0.3 13.3 1.6 D441101400015 45.6 0.4 10.9 1.3 D441101400016 44.3 0.4 9.3 1.1 D441101400017 43.0 0.4 6.2 0.7 D441101400018 41.6 0.4 4.2 0.5 D441101400019 40.2 0.5 2.4 0.3 D441101400020 38.7 0.5 1.7 0.3 D441101400021 35.7 0.5 0.3 0.1 D441101400022 ENDDATA 12 0 D441101400023 ENDSUBENT 22 0 D441101499999 ENDENTRY 14 0 D441199999999