ENTRY D4229 20091105 D071D422900000001 SUBENT D4229001 20091105 D071D422900100001 BIB 15 61 D422900100002 TITLE Production of the therapeutic radioisotope 114mIn D422900100003 through the 116Cd(p,3n)114mIn reaction D422900100004 AUTHOR (A.Hermanne,F.Tarkanyi,S.Takacs,P.Vandenwinkel, D422900100005 R.Adamrebeles,A.Ignatyuk,S.F.Kovalev) D422900100006 INSTITUTE (2BLGVUB,3HUNDEB,4RUSFEI) D422900100007 REFERENCE (J,ARI,68,14,2010) in press D422900100008 #doi:10.1016/j.apradiso.2009.08.014 D422900100009 SAMPLE Enriched 116Cd (97.4% 116Cd, 1.5% 114Cd,rest other D422900100010 stable Cd isotopes) D422900100011 FACILITY (CYCLO,2BLGVUB) D422900100012 DETECTOR (HPGE) D422900100013 METHOD Two stacks containing, respectively,16 and 11 D422900100014 enriched 116Cd targets(97.4% 116Cd, 1.5% 114Cd, rest D422900100015 other stable Cd isotopes) were irradiated in the D422900100016 external 37 and 16 MeV proton beams att he VUB D422900100017 cyclotron. The targets were prepared by D422900100018 electrodeposition on thin Cu strips (Goodfellow, D422900100019 thickness 12.3 microns) from analkaline bath containingD422900100020 1g enriched 116Cd. Electro deposition is done by D422900100021 means of controlled cathode potential electrolysis D422900100022 at 1.75 V versus amercury/ mercuroussulphate D422900100023 reference electrode. D422900100024 Irradiations took place in a Faraday-cup like target D422900100025 holder. The beam current was kept constant at D422900100026 approximately 150 nA during the 1500 s irradiation runsD422900100027 Decay characteristics for the studied isotopes were D422900100028 taken from NUDAT2 except for 114mIn where the data fromD422900100029 Browne and Firestone(1986) are used. D422900100030 For energy degradation in the stack foils a code based D422900100031 on polynomial approximations for the stopping powers D422900100032 of the elements present was used. D422900100033 MONITOR (29-CU-0(P,X)30-ZN-62,,SIG) D422900100034 (29-CU-0(P,X)30-ZN-65,,SIG) D422900100035 MONIT-REF (,S.TAKACS+,J,NIM/B,188,106,2002) D422900100036 (,F.TARKANYI+,R,IAEA-NDS-1211,2001) Chapter 4 D422900100037 DECAY-DATA Decay data were taken from NuDat database. D422900100038 ERR-ANALYS (EN-ERR)The incident energies were estimated at D422900100039 36.8 and 16.0 MeV with an uncertainty of +-0.1 MeV. D422900100040 Uncertainty on the median energy in each foil is D422900100041 increasing along the stack due to the cumulative D422900100042 effect of energy spread and variations in foils D422900100043 thickness and reaches a maximum of +-2 MeV for D422900100044 the last foil. D422900100045 (ERR-T) The uncertainties regarding cross section D422900100046 values were estimated according to the prescriptions D422900100047 of the ISO (1993) guidelines and obtained by quadratic D422900100048 summation of the individual contributions. D422900100049 (ERR-1)number of target nuclei (5%); D422900100050 (ERR-2)beam current (5%); D422900100051 (ERR-3,8.,10.)detector efficiency (8-10%) D422900100052 (ERR-4,1.,5.)statistical error and peak area fit (1-5%)D422900100053 (ERR-5,1.,5.) gamma-ray abundances(1-5%). D422900100054 ADD-RES (THEO) The experimental data were compared to the D422900100055 results of the theoretical model code ALICE-IPPE and D422900100056 EMPIRE model codes. D422900100057 (COMP) The measured experimental data were compared to D422900100058 those found in the literature. D422900100059 (TTY-C) Fitted excitation functions were used for D422900100060 determination of integral physical yields. D422900100061 STATUS (APRVD) S.Takacs, 2009.11.07. D422900100062 HISTORY (20091105C) TS. D422900100063 ENDBIB 61 0 D422900100064 COMMON 2 3 D422900100065 ERR-1 ERR-2 D422900100066 PER-CENT PER-CENT D422900100067 5. 5. D422900100068 ENDCOMMON 3 0 D422900100069 ENDSUBENT 68 0 D422900199999 SUBENT D4229002 20091105 D071D422900200001 BIB 3 3 D422900200002 REACTION (48-CD-116(P,4N)49-IN-113-M,,SIG) D422900200003 DECAY-DATA (49-IN-113-M,1.66HR,DG,391.7,0.649) D422900200004 STATUS (TABLE) Table 2 of reference. D422900200005 ENDBIB 3 0 D422900200006 NOCOMMON 0 0 D422900200007 DATA 4 10 D422900200008 EN EN-ERR DATA ERR-T D422900200009 MEV MEV MB MB D422900200010 36.8 0.1 83.2 7.0 D422900200011 35.7 0.2 74.1 6.0 D422900200012 34.5 0.2 61.2 5.0 D422900200013 33.4 0.3 56.1 4.0 D422900200014 32.2 0.4 48.0 4.0 D422900200015 31.0 0.5 33.1 3.0 D422900200016 29.7 0.6 19.3 2.0 D422900200017 28.4 0.7 6.4 1.0 D422900200018 27.0 0.8 1.9 0.3 D422900200019 25.6 0.9 1.0 0.2 D422900200020 ENDDATA 12 0 D422900200021 ENDSUBENT 20 0 D422900299999 SUBENT D4229003 20091105 D071D422900300001 BIB 3 4 D422900300002 REACTION (48-CD-116(P,3N)49-IN-114-M,,SIG) D422900300003 DECAY-DATA (49-IN-114-M,49.5D,DG,190.3,0.156,DG,558.4,0.044, D422900300004 DG,725.2,0.043) D422900300005 STATUS (TABLE) Table 2 of reference. D422900300006 ENDBIB 4 0 D422900300007 NOCOMMON 0 0 D422900300008 DATA 4 15 D422900300009 EN EN-ERR DATA ERR-T D422900300010 MEV MEV MB MB D422900300011 36.8 0.1 293.7 23.0 D422900300012 35.7 0.2 318.1 25.0 D422900300013 34.5 0.2 332.4 27.0 D422900300014 33.4 0.3 418.0 33.0 D422900300015 32.2 0.4 518.9 42.0 D422900300016 31.0 0.5 578.6 46.0 D422900300017 29.7 0.6 671.6 54.0 D422900300018 28.4 0.7 727.1 58.0 D422900300019 27.0 0.8 730.5 58.0 D422900300020 25.6 0.9 719.9 58.0 D422900300021 24.2 1.0 572.7 46.0 D422900300022 22.6 1.2 434.6 35.0 D422900300023 21.0 1.4 230.1 18.0 D422900300024 19.3 1.6 53.6 4.0 D422900300025 17.4 1.8 0.3 0.1 D422900300026 ENDDATA 17 0 D422900300027 ENDSUBENT 26 0 D422900399999 SUBENT D4229004 20091105 D071D422900400001 BIB 3 3 D422900400002 REACTION (48-CD-116(P,2N)49-IN-115-M,,SIG) D422900400003 DECAY-DATA (49-IN-115-M,4.48HR,DG,336.2,0.458) D422900400004 STATUS (TABLE) Table 2 of reference. D422900400005 ENDBIB 3 0 D422900400006 NOCOMMON 0 0 D422900400007 DATA 4 23 D422900400008 EN EN-ERR DATA ERR-T D422900400009 MEV MEV MB MB D422900400010 36.8 0.1 33.8 3.0 D422900400011 35.7 0.2 32.5 3.0 D422900400012 34.5 0.2 32.8 3.0 D422900400013 33.4 0.3 31.0 2.0 D422900400014 32.2 0.4 36.9 3.0 D422900400015 31.0 0.5 40.4 3.0 D422900400016 29.7 0.6 41.5 3.0 D422900400017 28.4 0.7 44.7 4.0 D422900400018 27.0 0.8 51.1 4.0 D422900400019 25.6 0.9 68.8 6.0 D422900400020 24.2 1.0 78.6 6.0 D422900400021 22.6 1.2 111.9 9.0 D422900400022 21.0 1.4 157.4 13.0 D422900400023 19.3 1.6 205.7 16.0 D422900400024 17.4 1.8 265.0 21.0 D422900400025 15.8 0.1 268.0 21.0 D422900400026 15.4 2.0 245.9 20.0 D422900400027 14.4 0.2 257.8 21.0 D422900400028 12.8 0.3 296.8 24.0 D422900400029 11.0 0.4 220.0 18.0 D422900400030 9.1 0.4 28.9 3.0 D422900400031 8.2 0.5 1.0 0.1 D422900400032 7.4 0.6 0.03 0.01 D422900400033 ENDDATA 25 0 D422900400034 ENDSUBENT 33 0 D422900499999 SUBENT D4229005 20091105 D071D422900500001 BIB 3 4 D422900500002 REACTION (48-CD-116(P,N)49-IN-116-M1+M2,,SIG) D422900500003 DECAY-DATA (49-IN-116-M1,54.4MIN,DG,416.9,0.277,DG,818.7,0.115, D422900500004 DG,1097.3,0.562,DG,1293.6,0.844) D422900500005 STATUS (TABLE) Table 2 of reference. D422900500006 ENDBIB 4 0 D422900500007 NOCOMMON 0 0 D422900500008 DATA 4 27 D422900500009 EN EN-ERR DATA ERR-T D422900500010 MEV MEV MB MB D422900500011 36.8 0.1 13.1 1.0 D422900500012 35.7 0.2 13.3 1.0 D422900500013 34.5 0.2 12.6 1.0 D422900500014 33.4 0.3 12.4 1.0 D422900500015 32.2 0.4 13.4 1.0 D422900500016 31.0 0.5 13.8 1.0 D422900500017 29.7 0.6 15.4 1.0 D422900500018 28.4 0.7 17.1 1.0 D422900500019 27.0 0.8 16.2 1.0 D422900500020 25.6 0.9 18.5 1.0 D422900500021 24.2 1.0 18.3 1.0 D422900500022 22.6 1.2 20.9 2.0 D422900500023 21.0 1.4 20.5 2.0 D422900500024 19.3 1.6 21.1 2.0 D422900500025 17.4 1.8 26.5 2.0 D422900500026 15.8 0.1 26.0 2.0 D422900500027 15.4 2.0 30.0 2.0 D422900500028 14.4 0.2 32.7 3.0 D422900500029 12.8 0.3 65.9 5.0 D422900500030 11.0 0.4 108.6 9.0 D422900500031 9.1 0.4 169.5 14.0 D422900500032 8.2 0.5 140.0 11.0 D422900500033 7.4 0.6 92.7 7.0 D422900500034 6.4 0.8 42.3 3.0 D422900500035 5.3 1.0 13.7 1.0 D422900500036 4.1 1.3 2.0 0.3 D422900500037 2.5 1.6 0.2 0.03 D422900500038 ENDDATA 29 0 D422900500039 ENDSUBENT 38 0 D422900599999 SUBENT D4229006 20091105 D071D422900600001 BIB 3 4 D422900600002 REACTION (48-CD-116(P,X)48-CD-115-G,,SIG) D422900600003 DECAY-DATA (48-CD-115-G,53.5HR,DG,336.2,0.459,DG,492.4,0.08, D422900600004 DG,527.9,0.275) D422900600005 STATUS (TABLE) Table 2 of reference. D422900600006 ENDBIB 4 0 D422900600007 NOCOMMON 0 0 D422900600008 DATA 4 19 D422900600009 EN EN-ERR DATA ERR-T D422900600010 MEV MEV MB MB D422900600011 36.8 0.1 104.9 8.0 D422900600012 35.7 0.2 96.6 8.0 D422900600013 34.5 0.2 85.9 7.0 D422900600014 33.4 0.3 88.8 7.0 D422900600015 32.2 0.4 99.0 8.0 D422900600016 31.0 0.5 92.1 7.0 D422900600017 29.7 0.6 94.2 8.0 D422900600018 28.4 0.7 96.5 8.0 D422900600019 27.0 0.8 90.2 7.0 D422900600020 25.6 0.9 96.8 8.0 D422900600021 24.2 1.0 79.1 6.0 D422900600022 22.6 1.2 73.9 6.0 D422900600023 21.0 1.4 61.5 5.0 D422900600024 19.3 1.6 46.4 4.0 D422900600025 17.4 1.8 36.1 3.0 D422900600026 15.8 0.1 16.7 1.0 D422900600027 15.4 2.0 19.0 2.0 D422900600028 14.4 0.2 8.8 1.0 D422900600029 12.8 0.3 2.6 0.5 D422900600030 ENDDATA 21 0 D422900600031 ENDSUBENT 30 0 D422900699999 ENDENTRY 6 0 D422999999999