ENTRY D0967 20200603 D127D096700000001 SUBENT D0967001 20200603 D127D096700100001 BIB 13 45 D096700100002 TITLE Measurement of cross-sections of proton-induced D096700100003 nuclear reactions on 197Au focused on the production D096700100004 of the theranostic pair 197m,gHg D096700100005 AUTHOR (J.Cervenak, O.Lebeda) D096700100006 INSTITUTE (3CZRUJF) D096700100007 REFERENCE (J,NIM/B,458,118,2019) D096700100008 (J,NIM/B,478,85,2020) Revised 197m,gHg production data D096700100009 FACILITY (ISOCY,3CZRUJF) U-120M cyclotron D096700100010 SAMPLE Au foils (99.9% purity, 7 um thick), D096700100011 Ti foils (99.6% purity, 11.0 um thick), D096700100012 Cu foils (55.9 and 10.6 um thick) D096700100013 DETECTOR (HPGE) Calibrated using a set of point-like 241Am, D096700100014 152Eu, 137Cs, 133Ba and 60Co standards D096700100015 METHOD (EXTB) D096700100016 (BCINT) The recorded beam current value and incident D096700100017 energies were slightly corrected by reconstruction of D096700100018 the Ti(p,x)48V IAEA monitor excitation function. D096700100019 The Ti monitors were measured after ca 16 days to D096700100020 avoid the interference from the 48Sc decay gammas. D096700100021 The 48V activity fractions ejected from the monitor D096700100022 foil to the following Au foil were measured and D096700100023 added to the activity measured in the monitor itself D096700100024 (0.5-3.5% of 48V). D096700100025 (STTA) Two stacks were irradiated. D096700100026 Stack 1: 13 Au foils and 14 Ti foils interleaved with D096700100027 thicker Cu degraders bombarded with proton at D096700100028 35.2+/-0.2 MeV. D096700100029 Stack 2: 12 Au foils and 12 Ti foils interleaved with D096700100030 thinner Cu degraders bombarded with proton at D096700100031 17.3+/-0.2 MeV. D096700100032 (ACTIV) Irradiated for 1 hr D096700100033 REL-REF (R,,K.Gul+,R,IAEA-TECDOC-1211,2001) D096700100034 Ti(p,x)48V IAEA monitor cross section D096700100035 ADD-RES (TTY-C) Thick target yield from the measured cross D096700100036 sections D096700100037 ERR-ANALYS (EN-ERR) Uncertainty in the initial beam energy D096700100038 (ERR-T) Total uncertainty was deduced from D096700100039 Gamma emission probability (usually <5%) D096700100040 (ERR-1) gamma detection efficiency (~3%) D096700100041 (ERR-2,,10.) net peak area (<10%) D096700100042 (ERR-3) beam current (~6%) D096700100043 (ERR-4,,2.) foil thickness (<2%) D096700100044 STATUS (APRVD) Proofread by O.Lebeda (2020-01-21, 2020-06-03) D096700100045 HISTORY (20200111C) On D096700100046 (20200603A) On. 009-010 added. D096700100047 ENDBIB 45 0 D096700100048 COMMON 3 3 D096700100049 EN-ERR ERR-1 ERR-3 D096700100050 MEV PER-CENT PER-CENT D096700100051 0.2 3. 6. D096700100052 ENDCOMMON 3 0 D096700100053 ENDSUBENT 52 0 D096700199999 SUBENT D0967002 20200603 D127D096700200001 BIB 4 5 D096700200002 REACTION (79-AU-197(P,N)80-HG-197-M,,SIG) D096700200003 DECAY-DATA (80-HG-197-M,23.8HR,DG,133.98,0.335) D096700200004 STATUS (TABLE) Table 2 of Nucl.Instrum.Meth.B458(2019)118 D096700200005 (SPSDD,D0967009) Decay data updated D096700200006 HISTORY (20200603U) On. STATUS updated. D096700200007 ENDBIB 5 0 D096700200008 NOCOMMON 0 0 D096700200009 DATA 4 25 D096700200010 EN EN-RSL-HW DATA ERR-T D096700200011 MEV MEV MB MB D096700200012 35.29 0.20 8.10 0.56 D096700200013 34.07 0.20 8.33 0.58 D096700200014 32.81 0.20 8.72 0.61 D096700200015 31.51 0.21 8.85 0.62 D096700200016 30.17 0.21 9.20 0.64 D096700200017 28.77 0.22 9.57 0.67 D096700200018 27.35 0.22 11.45 0.79 D096700200019 25.86 0.23 11.42 0.79 D096700200020 24.30 0.23 12.16 0.84 D096700200021 22.65 0.24 11.31 0.78 D096700200022 20.90 0.25 9.77 0.67 D096700200023 19.03 0.27 12.70 0.87 D096700200024 17.32 0.20 14.2 1.0 D096700200025 17.04 0.28 14.3 1.0 D096700200026 16.08 0.20 15.3 1.1 D096700200027 14.79 0.21 18.1 1.2 D096700200028 13.41 0.22 24.9 1.7 D096700200029 12.66 0.23 30.2 2.1 D096700200030 11.87 0.23 37.6 2.6 D096700200031 11.05 0.24 35.6 2.4 D096700200032 10.19 0.25 30.3 2.1 D096700200033 9.27 0.26 19.2 1.3 D096700200034 8.28 0.27 8.27 0.57 D096700200035 7.19 0.30 2.07 0.14 D096700200036 6.35 0.32 0.504 0.037 D096700200037 ENDDATA 27 0 D096700200038 ENDSUBENT 37 0 D096700299999 SUBENT D0967003 20200603 D127D096700300001 BIB 5 6 D096700300002 REACTION (79-AU-197(P,N)80-HG-197-G,,SIG) D096700300003 DECAY-DATA (80-HG-197-G,64.14HR,DG,191.437,0.00632) D096700300004 CORRECTION Corrected for 197mHg decay contribution D096700300005 STATUS (TABLE) Table 2 of Nucl.Instrum.Meth.B458(2019)118 D096700300006 (SPSDD,D0967010) Decay data and uncertainty updated D096700300007 HISTORY (20200603U) On. STATUS updated. D096700300008 ENDBIB 6 0 D096700300009 NOCOMMON 0 0 D096700300010 DATA 4 19 D096700300011 EN EN-RSL-HW DATA ERR-T D096700300012 MEV MEV MB MB D096700300013 27.35 0.22 12.1 2.1 D096700300014 25.86 0.23 10.7 3.4 D096700300015 24.30 0.23 12.0 3.3 D096700300016 22.65 0.24 12.5 3.0 D096700300017 20.90 0.25 13.5 2.2 D096700300018 19.03 0.27 15.7 1.7 D096700300019 17.32 0.20 17.4 1.2 D096700300020 17.04 0.28 16.0 1.7 D096700300021 16.08 0.20 19.4 1.4 D096700300022 14.79 0.21 22.5 1.6 D096700300023 13.41 0.22 35.6 2.5 D096700300024 12.66 0.23 42.8 3.0 D096700300025 11.87 0.23 57.4 4.0 D096700300026 11.05 0.24 62.5 4.4 D096700300027 10.19 0.25 65.7 4.6 D096700300028 9.27 0.26 57.3 4.0 D096700300029 8.28 0.27 30.2 2.1 D096700300030 7.19 0.30 8.34 0.63 D096700300031 6.35 0.32 2.02 0.21 D096700300032 ENDDATA 21 0 D096700300033 ENDSUBENT 32 0 D096700399999 SUBENT D0967004 20200603 D127D096700400001 BIB 4 4 D096700400002 REACTION (79-AU-197(P,3N)80-HG-195-M,,SIG) D096700400003 DECAY-DATA (80-HG-195-M,41.6HR,DG,560.27,0.071) D096700400004 STATUS (TABLE) Table 2 of Nucl.Instrum.Meth.B458(2019)118 D096700400005 HISTORY (20200603U) On. STATUS moved from 001. D096700400006 ENDBIB 4 0 D096700400007 NOCOMMON 0 0 D096700400008 DATA 4 13 D096700400009 EN EN-RSL-HW DATA ERR-T D096700400010 MEV MEV MB MB D096700400011 35.29 0.20 243. 17. D096700400012 34.07 0.20 321. 22. D096700400013 32.81 0.20 428. 29. D096700400014 31.51 0.21 554. 38. D096700400015 30.17 0.21 693. 48. D096700400016 28.77 0.22 760. 52. D096700400017 27.35 0.22 779. 54. D096700400018 25.86 0.23 703. 48. D096700400019 24.30 0.23 603. 42. D096700400020 22.65 0.24 458. 32. D096700400021 20.90 0.25 250. 17. D096700400022 19.03 0.27 51.6 2.4 D096700400023 17.04 0.28 0.56 0.19 D096700400024 ENDDATA 15 0 D096700400025 ENDSUBENT 24 0 D096700499999 SUBENT D0967005 20200603 D127D096700500001 BIB 5 5 D096700500002 REACTION (79-AU-197(P,3N)80-HG-195-G,,SIG) D096700500003 DECAY-DATA (80-HG-195-G,10.53HR,DG,779.80,0.070) D096700500004 CORRECTION Corrected for 195mHg decay contribution D096700500005 STATUS (TABLE) Table 2 of Nucl.Instrum.Meth.B458(2019)118 D096700500006 HISTORY (20200603U) On. STATUS moved from 001. D096700500007 ENDBIB 5 0 D096700500008 NOCOMMON 0 0 D096700500009 DATA 4 13 D096700500010 EN EN-RSL-HW DATA ERR-T D096700500011 MEV MEV MB MB D096700500012 35.29 0.20 90.6 6.3 D096700500013 34.07 0.20 109.7 7.6 D096700500014 32.81 0.20 174. 12. D096700500015 31.51 0.21 233. 16. D096700500016 30.17 0.21 315. 22. D096700500017 28.77 0.22 390. 27. D096700500018 27.35 0.22 449. 31. D096700500019 25.86 0.23 427. 29. D096700500020 24.30 0.23 402. 28. D096700500021 22.65 0.24 344. 24. D096700500022 20.90 0.25 216. 15. D096700500023 19.03 0.27 54.5 1.1 D096700500024 17.04 0.28 1.12 0.44 D096700500025 ENDDATA 15 0 D096700500026 ENDSUBENT 25 0 D096700599999 SUBENT D0967006 20200603 D127D096700600001 BIB 4 4 D096700600002 REACTION (79-AU-197(P,X)79-AU-196-M2,,SIG) D096700600003 DECAY-DATA (79-AU-196-M2,9.6HR,DG,147.81,0.435) D096700600004 STATUS (TABLE) Table 2 of Nucl.Instrum.Meth.B458(2019)118 D096700600005 HISTORY (20200603U) On. STATUS moved from 001. D096700600006 ENDBIB 4 0 D096700600007 NOCOMMON 0 0 D096700600008 DATA 4 14 D096700600009 EN EN-RSL-HW DATA ERR-T D096700600010 MEV MEV MB MB D096700600011 35.29 0.20 9.18 0.63 D096700600012 34.07 0.20 9.02 0.62 D096700600013 32.81 0.20 8.52 0.59 D096700600014 31.51 0.21 7.99 0.55 D096700600015 30.17 0.21 7.32 0.51 D096700600016 28.77 0.22 6.32 0.44 D096700600017 27.35 0.22 5.40 0.37 D096700600018 25.86 0.23 4.25 0.29 D096700600019 24.30 0.23 2.97 0.21 D096700600020 22.65 0.24 1.72 0.12 D096700600021 20.90 0.25 0.781 0.060 D096700600022 19.03 0.27 0.254 0.021 D096700600023 17.32 0.20 0.0188 0.022 D096700600024 17.04 0.28 0.134 0.010 D096700600025 ENDDATA 16 0 D096700600026 ENDSUBENT 25 0 D096700699999 SUBENT D0967007 20200603 D127D096700700001 BIB 5 5 D096700700002 REACTION (79-AU-197(P,X)79-AU-196-G+M1,,SIG) D096700700003 DECAY-DATA (79-AU-196-G,6.1669D,DG,355.73,0.87) D096700700004 CORRECTION Corrected for 196m2Au decay contribution D096700700005 STATUS (TABLE) Table 2 of Nucl.Instrum.Meth.B458(2019)118 D096700700006 HISTORY (20200603U) On. STATUS moved from 001. D096700700007 ENDBIB 5 0 D096700700008 NOCOMMON 0 0 D096700700009 DATA 4 18 D096700700010 EN EN-RSL-HW DATA ERR-T D096700700011 MEV MEV MB MB D096700700012 35.29 0.20 158. 11. D096700700013 34.07 0.20 159. 11. D096700700014 32.81 0.20 158. 11. D096700700015 31.51 0.21 154. 11. D096700700016 30.17 0.21 152. 10. D096700700017 28.77 0.22 145. 10. D096700700018 27.35 0.22 138.1 9.5 D096700700019 25.86 0.23 125.2 8.7 D096700700020 24.30 0.23 106.5 7.5 D096700700021 22.65 0.24 86.4 6.1 D096700700022 20.90 0.25 64.5 5.0 D096700700023 19.03 0.27 34.0 2.9 D096700700024 17.32 0.20 18.9 2.2 D096700700025 17.04 0.28 17.9 1.3 D096700700026 16.08 0.20 9.56 0.66 D096700700027 14.79 0.21 3.28 0.23 D096700700028 13.41 0.22 0.607 0.043 D096700700029 12.66 0.23 0.186 0.015 D096700700030 ENDDATA 20 0 D096700700031 ENDSUBENT 30 0 D096700799999 SUBENT D0967008 20200603 D127D096700800001 BIB 4 4 D096700800002 REACTION (79-AU-197(P,X)79-AU-194,,SIG) D096700800003 DECAY-DATA (79-AU-194-G,38.02HR,DG,328.464,0.604) D096700800004 STATUS (TABLE) Table 2 of Nucl.Instrum.Meth.B458(2019)118 D096700800005 HISTORY (20200603U) On. STATUS moved from 001. D096700800006 ENDBIB 4 0 D096700800007 NOCOMMON 0 0 D096700800008 DATA 4 10 D096700800009 EN EN-RSL-HW DATA ERR-T D096700800010 MEV MEV MB MB D096700800011 35.29 0.20 10.84 0.76 D096700800012 34.07 0.20 7.48 0.53 D096700800013 32.81 0.20 5.27 0.38 D096700800014 31.51 0.21 3.81 0.28 D096700800015 30.17 0.21 2.68 0.20 D096700800016 28.77 0.22 1.78 0.14 D096700800017 27.35 0.22 1.23 0.10 D096700800018 25.86 0.23 1.12 0.10 D096700800019 24.30 0.23 0.480 0.056 D096700800020 22.65 0.24 0.226 0.041 D096700800021 ENDDATA 12 0 D096700800022 ENDSUBENT 21 0 D096700899999 SUBENT D0967009 20200603 D127D096700900001 BIB 4 4 D096700900002 REACTION (79-AU-197(P,N)80-HG-197-M,,SIG) D096700900003 DECAY-DATA (80-HG-197-M,23.82HR,DG,133.79,0.348) D096700900004 STATUS (TABLE) Table 2 of Nucl.Instrum.Meth.B478(2020)85 D096700900005 HISTORY (20200603C) On D096700900006 ENDBIB 4 0 D096700900007 NOCOMMON 0 0 D096700900008 DATA 4 25 D096700900009 EN EN-RSL-HW DATA ERR-T D096700900010 MEV MEV MB MB D096700900011 35.29 0.20 7.80 0.54 D096700900012 34.07 0.20 8.03 0.56 D096700900013 32.81 0.20 8.39 0.59 D096700900014 31.51 0.21 8.53 0.60 D096700900015 30.17 0.21 8.86 0.62 D096700900016 28.77 0.22 9.20 0.65 D096700900017 27.35 0.22 9.53 0.66 D096700900018 25.86 0.23 10.98 0.77 D096700900019 24.30 0.23 10.10 0.70 D096700900020 22.65 0.24 10.89 0.76 D096700900021 20.90 0.25 11.68 0.81 D096700900022 19.03 0.27 12.23 0.85 D096700900023 17.32 0.20 13.66 0.95 D096700900024 17.04 0.28 13.79 0.96 D096700900025 16.08 0.20 14.74 1.0 D096700900026 14.79 0.21 17.4 1.2 D096700900027 13.41 0.22 24.0 1.7 D096700900028 12.66 0.23 29.0 2.0 D096700900029 11.87 0.23 36.2 2.5 D096700900030 11.05 0.24 34.3 2.4 D096700900031 10.19 0.25 29.1 2.0 D096700900032 9.27 0.26 18.4 1.3 D096700900033 8.28 0.27 7.95 0.55 D096700900034 7.19 0.30 1.99 0.14 D096700900035 6.35 0.32 0.475 0.035 D096700900036 ENDDATA 27 0 D096700900037 ENDSUBENT 36 0 D096700999999 SUBENT D0967010 20200603 D127D096701000001 BIB 5 5 D096701000002 REACTION (79-AU-197(P,N)80-HG-197-G,,SIG) D096701000003 DECAY-DATA (80-HG-197-G,64.81HR,DG,191.437,0.00632) D096701000004 CORRECTION Corrected for 197mHg decay contribution D096701000005 STATUS (TABLE) Table 2 of Nucl.Instrum.Meth.B478(2020)85 D096701000006 HISTORY (20200603C) On D096701000007 ENDBIB 5 0 D096701000008 NOCOMMON 0 0 D096701000009 DATA 4 19 D096701000010 EN EN-RSL-HW DATA ERR-T D096701000011 MEV MEV MB MB D096701000012 27.35 0.22 13.7 3.7 D096701000013 25.86 0.23 10.9 5.2 D096701000014 24.30 0.23 13.1 5.2 D096701000015 22.65 0.24 12.7 4.6 D096701000016 20.90 0.25 13.7 3.3 D096701000017 19.03 0.27 15.3 1.9 D096701000018 17.32 0.20 17.6 1.4 D096701000019 17.04 0.28 16.2 1.8 D096701000020 16.08 0.20 19.6 1.7 D096701000021 14.79 0.21 22.7 2.3 D096701000022 13.41 0.22 35.9 3.3 D096701000023 12.66 0.23 43.2 3.0 D096701000024 11.87 0.23 58.1 3.9 D096701000025 11.05 0.24 63.2 4.5 D096701000026 10.19 0.25 66.4 5.3 D096701000027 9.27 0.26 57.9 4.5 D096701000028 8.28 0.27 30.5 2.4 D096701000029 7.19 0.30 10.22 0.88 D096701000030 6.35 0.32 2.02 0.26 D096701000031 ENDDATA 21 0 D096701000032 ENDSUBENT 31 0 D096701099999 ENDENTRY 10 0 D096799999999