ENTRY 33106 20181230 31883310600000001 SUBENT 33106001 20181230 31883310600100001 BIB 11 61 3310600100002 TITLE Charge distribution of light mass fission products in 3310600100003 the fast neutron induced fission of 232Th, 238U, 240Pu 3310600100004 and 244Cm 3310600100005 AUTHOR (Haladhara Naik, Ram Janam Singh, 3310600100006 Shrikant Pandurang Dange) 3310600100007 INSTITUTE (3INDTRM) 3310600100008 REFERENCE (J,ARI,127,92,2017) 3310600100009 REL-REF (R,22119002,M.Haddad+,J,RCA,46,23,1989) 3310600100010 Nuclear spectroscopic data 3310600100011 (R,22134002,A.Srivastava+,J,RCA,46,17,1989) 3310600100012 Nuclear spectroscopic data 3310600100013 (N,,H.Naik+,J,EPJ/A,16,495,2003) 3310600100014 Mean neutron energy value given 3310600100015 (R,,B.F.Rider,R,NEDO-12154-3C,1981) 3310600100016 Adopted chain yields given 3310600100017 FACILITY (REAC,3INDTRM) Highly enriched uranium-fuelled light- 3310600100018 water-moderated swimming pool reactor APSARA, for 3310600100019 long-lived fission products 3310600100020 Heavy-water-moderated natural uranium-fuelled CIRUS, 3310600100021 for short-lived fission products. 3310600100022 SAMPLE For long-lived fission products: 3310600100023 232Th: 25 um thick metal foil (50 mg) wrapped with a 3310600100024 75 um thick Lexan foil 3310600100025 238U: Electrodeposited target of 99.9997 atom % 3310600100026 (~500 ug) 3310600100027 240Pu: Electrodeposited target of 99.48 atom % (96 ug) 3310600100028 244Cm: Electrodeposited target of 99.43 atom % (96 ug) 3310600100029 These were covered with a 75 um thick Lexan foils. The 3310600100030 Lexan foil act as catcher to collect the recoiling 3310600100031 fission products. The individual samples were wrapped 3310600100032 with 1 mm thick Cd foil, doubly sealed in alkathene 3310600100033 bags. 3310600100034 For short-lived fission products: 3310600100035 232Th: ~200 uL (50 mg/mL) 3310600100036 238U: ~200 uL (30 mg/mL) 3310600100037 240Pu: ~200 uL (0.507 mg/mL) 3310600100038 244Cm: ~200 uL (0.55 mg/mL) 3310600100039 Nitrate solutions were sealed in different 3310600100040 polypropylene tubes, covered with 1 mm thick Cd foils 3310600100041 and doubly sealed in alkathene bags. 3310600100042 DETECTOR (HPGE) 120 cm3 HPGE detector coupled to a 4096 PC- 3310600100043 based channel analyzer for long lived fission products.3310600100044 The efficiency and resolution of the detector was 20% 3310600100045 and 1.8 keV at energy 1332.5 keV. 3310600100046 (HPGE) 80 cm3 HPGE detector coupled to a 4096 PC- 3310600100047 based channel analyzer for short lived fission 3310600100048 products. The resolution of the detector was 2.0 keV 3310600100049 at 1332.5 keV and dead time of detector always kept 3310600100050 less than 10%. 3310600100051 METHOD (ACTIV) Long-lived fission products reactions were 3310600100052 irradiated for 5-60 min. 3310600100053 The short-lived fission products reactions for 1-5 min 3310600100054 with pneumatic carrier facility. 3310600100055 ERR-ANALYS (DATA-ERR) The uncertainties shown on FCY values for 3310600100056 fission products such as 89,90Kr, 93,94Sr, 95Y, 103Mo, 3310600100057 105,106Tc and 108Ru are propagated errors due to 3310600100058 uncertainties on cumulative yields and the mass chain 3310600100059 yields. The uncertainties of the fission products such 3310600100060 as 91,92Sr, 97Zr and 112Pd are due to replicate 3310600100061 measurements using the parent-daughter genetic relation3310600100062 HISTORY (20181230C) Gulshan Premi and VT 3310600100063 ENDBIB 61 0 3310600100064 COMMON 1 3 3310600100065 EN-MEAN 3310600100066 MEV 3310600100067 1.9 3310600100068 ENDCOMMON 3 0 3310600100069 ENDSUBENT 68 0 3310600199999 SUBENT 33106002 20181230 31883310600200001 BIB 6 8 3310600200002 REACTION (90-TH-232(N,F)ELEM/MASS,CUM,FY,,FRC/SPA) 3310600200003 DECAY-DATA ((1.)38-SR-94,75.3SEC,DG,1427.7,0.942) 3310600200004 ((2.)40-ZR-97,16.749HR,DG,743.4,0.9399) 3310600200005 MONITOR (90-TH-232(N,F)40-ZR-97,CUM,FY,,SPA) 3310600200006 MONIT-REF (,H.N.Erten+,J,NSE,79,167,1981) 3310600200007 ANALYSIS Measured cumulative yield divided by the chain yield 3310600200008 in the literature 3310600200009 STATUS (TABLE) Table 2 of Applied Rad. Isotopes, 127 (2017) 923310600200010 ENDBIB 8 0 3310600200011 NOCOMMON 0 0 3310600200012 DATA 5 2 3310600200013 ELEMENT MASS DATA DATA-ERR DECAY-FLAG 3310600200014 NO-DIM NO-DIM NO-DIM NO-DIM NO-DIM 3310600200015 38. 94. 0.989 0.014 1. 3310600200016 40. 97. 0.9995 0.0005 2. 3310600200017 ENDDATA 4 0 3310600200018 ENDSUBENT 17 0 3310600299999 SUBENT 33106003 20181230 31883310600300001 BIB 6 9 3310600300002 REACTION (92-U-238(N,F)ELEM/MASS,CUM,FY,,FRC/SPA) 3310600300003 DECAY-DATA ((1.)38-SR-94,75.3SEC,DG,1427.7,0.942) 3310600300004 ((2.)40-ZR-97,16.749HR,DG,743.4,0.9399) 3310600300005 ((3.)42-MO-103,67.5SEC,DG,687.6,0.160) 3310600300006 MONITOR (92-U-238(N,F)40-ZR-97,CUM,FY,,SPA) 3310600300007 MONIT-REF (,R.H.Iyer+,J,NSE,135,1,2000) 3310600300008 ANALYSIS Measured cumulative yield divided by the chain yield 3310600300009 in the literature 3310600300010 STATUS (TABLE) Table 2 of Applied Rad. Isotopes, 127 (2017) 923310600300011 ENDBIB 9 0 3310600300012 NOCOMMON 0 0 3310600300013 DATA 5 3 3310600300014 ELEMENT MASS DATA DATA-ERR DECAY-FLAG 3310600300015 NO-DIM NO-DIM NO-DIM NO-DIM NO-DIM 3310600300016 38. 94. 0.990 0.017 1. 3310600300017 40. 97. 0.9995 0.0004 2. 3310600300018 42. 103. 0.995 0.015 3. 3310600300019 ENDDATA 5 0 3310600300020 ENDSUBENT 19 0 3310600399999 SUBENT 33106004 20181230 31883310600400001 BIB 6 17 3310600400002 REACTION (94-PU-240(N,F)ELEM/MASS,CUM,FY,,FRC/SPA) 3310600400003 DECAY-DATA ((1.)36-KR-89,3.15MIN,DG,586.0,0.167) 3310600400004 ((2.)38-SR-91,9.63HR,DG,749.8,0.237) 3310600400005 ((3.)38-SR-92,2.66HR,DG,1383.9,0.900) 3310600400006 ((4.)38-SR-93,7.43MIN,DG,590.2,0.680) 3310600400007 ((5.)38-SR-94,75.3SEC,DG,1427.7,0.942) 3310600400008 ((6.)39-Y-95,10.3MIN,DG,954.1,0.158) 3310600400009 ((7.)40-ZR-97,16.749HR,DG,743.4,0.9399) 3310600400010 ((8.)42-MO-103,67.5SEC,DG,687.6,0.160) 3310600400011 ((9.)43-TC-105,7.6MIN,DG,143.3,0.157) 3310600400012 ((10.)43-TC-106,35.6SEC,DG,270.1,0.558) 3310600400013 ((11.)44-RU-108,4.55MIN,DG,164.9,0.280) 3310600400014 MONITOR (94-PU-240(N,F)40-ZR-97,CUM,FY,,SPA) 3310600400015 MONIT-REF (,R.H.Iyer+,J,NSE,135,1,2000) 3310600400016 STATUS (TABLE) Table 2 of Applied Rad. Isotopes, 127 (2017) 923310600400017 ANALYSIS Measured cumulative yield divided by the chain yield 3310600400018 in the literature 3310600400019 ENDBIB 17 0 3310600400020 NOCOMMON 0 0 3310600400021 DATA 5 11 3310600400022 ELEMENT MASS DATA DATA-ERR DECAY-FLAG 3310600400023 NO-DIM NO-DIM NO-DIM NO-DIM NO-DIM 3310600400024 36. 89. 0.923 0.031 1. 3310600400025 38. 91. 0.9953 0.0045 2. 3310600400026 38. 92. 0.9828 0.0031 3. 3310600400027 38. 93. 0.945 0.025 4. 3310600400028 38. 94. 0.864 0.015 5. 3310600400029 39. 95. 0.985 0.005 6. 3310600400030 40. 97. 0.9862 0.0021 7. 3310600400031 42. 103. 0.935 0.038 8. 3310600400032 43. 105. 0.962 0.014 9. 3310600400033 43. 106. 0.897 0.041 10. 3310600400034 44. 108. 0.959 0.015 11. 3310600400035 ENDDATA 13 0 3310600400036 ENDSUBENT 35 0 3310600499999 SUBENT 33106005 20181230 31883310600500001 BIB 6 17 3310600500002 REACTION (96-CM-244(N,F)ELEM/MASS,CUM,FY,,FRC/SPA) 3310600500003 DECAY-DATA ((1.)36-KR-89,3.15MIN,DG,586.0,0.167) 3310600500004 ((2.)36-KR-90,32.32SEC,DG,539.5,0.308) 3310600500005 ((3.)38-SR-91,9.63HR,DG,749.8,0.237) 3310600500006 ((4.)38-SR-92,2.66HR,DG,1383.9,0.900) 3310600500007 ((5.)38-SR-93,7.43MIN,DG,590.2,0.680) 3310600500008 ((6.)38-SR-94,75.3SEC,DG,1427.7,0.942) 3310600500009 ((7.)39-Y-95,10.3MIN,DG,954.1,0.158) 3310600500010 ((8.)40-ZR-97,16.749HR,DG,743.4,0.9399) 3310600500011 ((9.)42-MO-103,67.5SEC,DG,687.6,0.160) 3310600500012 ((10.)43-TC-105,7.6MIN,DG,143.3,0.157) 3310600500013 ((11.)44-RU-108,4.55MIN,DG,164.9,0.280) 3310600500014 MONITOR (96-CM-244(N,F)40-ZR-97,CUM,FY,,SPA) 3310600500015 MONIT-REF (,R.H.Iyer+,J,NSE,135,1,2000) 3310600500016 ANALYSIS Measured cumulative yield divided by the chain yield 3310600500017 in the literature 3310600500018 STATUS (TABLE) Table 2 of Applied Rad. Isotopes, 127 (2017) 923310600500019 ENDBIB 17 0 3310600500020 NOCOMMON 0 0 3310600500021 DATA 5 12 3310600500022 ELEMENT MASS DATA DATA-ERR DECAY-FLAG 3310600500023 NO-DIM NO-DIM NO-DIM NO-DIM NO-DIM 3310600500024 36. 89. 0.802 0.027 1. 3310600500025 36. 90. 0.563 0.020 2. 3310600500026 38. 91. 0.984 0.004 3. 3310600500027 38. 92. 0.938 0.007 4. 3310600500028 38. 93. 0.862 0.046 5. 3310600500029 38. 94. 0.768 0.022 6. 3310600500030 39. 95. 0.952 0.037 7. 3310600500031 40. 97. 0.951 0.012 8. 3310600500032 42. 103. 0.891 0.044 9. 3310600500033 43. 105. 0.929 0.033 10. 3310600500034 44. 108. 0.901 0.026 11. 3310600500035 46. 112. 0.963 0.019 3310600500036 ENDDATA 14 0 3310600500037 ENDSUBENT 36 0 3310600599999 SUBENT 33106006 20181230 31883310600600001 BIB 4 6 3310600600002 REACTION (90-TH-232(N,F)MASS,,ZP,,SPA) 3310600600003 ANALYSIS Gaussian fitting without considering the even-odd 3310600600004 effect 3310600600005 STATUS (TABLE) Table 3 of Applied Rad. Isotopes, 127 (2017) 923310600600006 (DEP,33106002) Fractional cumulative yield 3310600600007 MISC-COL (MISC) Charge dispersion parameter 3310600600008 ENDBIB 6 0 3310600600009 NOCOMMON 0 0 3310600600010 DATA 4 8 3310600600011 MASS DATA DATA-ERR MISC 3310600600012 NO-DIM NO-DIM NO-DIM NO-DIM 3310600600013 85. 33.55 0.07 0.55 3310600600014 86. 34.00 0.13 0.57 3310600600015 89. 35.10 0.15 0.50 3310600600016 91. 36.00 0.05 0.50 3310600600017 92. 36.40 0.07 0.52 3310600600018 93. 36.70 0.05 0.52 3310600600019 94. 37.20 0.15 0.56 3310600600020 97. 38.60 0.11 0.57 3310600600021 ENDDATA 10 0 3310600600022 ENDSUBENT 21 0 3310600699999 SUBENT 33106007 20181230 31883310600700001 BIB 4 6 3310600700002 REACTION (92-U-238(N,F)MASS,,ZP,,SPA) 3310600700003 ANALYSIS Gaussian fitting without considering the even-odd 3310600700004 effect 3310600700005 STATUS (TABLE) Table 3 of Applied Rad. Isotopes, 127 (2017) 923310600700006 (DEP,33106003) Fractional cumulative yield 3310600700007 MISC-COL (MISC) Charge dispersion parameter 3310600700008 ENDBIB 6 0 3310600700009 NOCOMMON 0 0 3310600700010 DATA 4 7 3310600700011 MASS DATA DATA-ERR MISC 3310600700012 NO-DIM NO-DIM NO-DIM NO-DIM 3310600700013 89. 34.90 0.15 0.56 3310600700014 91. 35.80 0.09 0.63 3310600700015 92. 36.30 0.12 0.56 3310600700016 93. 36.75 0.12 0.58 3310600700017 94. 37.10 0.17 0.60 3310600700018 97. 38.50 0.12 0.60 3310600700019 103. 40.80 0.15 0.65 3310600700020 ENDDATA 9 0 3310600700021 ENDSUBENT 20 0 3310600799999 SUBENT 33106008 20181230 31883310600800001 BIB 4 6 3310600800002 REACTION (94-PU-240(N,F)MASS,,ZP,,SPA) 3310600800003 ANALYSIS Gaussian fitting without considering the even-odd 3310600800004 effect 3310600800005 STATUS (TABLE) Table 3 of Applied Rad. Isotopes, 127 (2017) 923310600800006 (DEP,33106004) Fractional cumulative yield 3310600800007 MISC-COL (MISC) Charge dispersion parameter 3310600800008 ENDBIB 6 0 3310600800009 NOCOMMON 0 0 3310600800010 DATA 4 11 3310600800011 MASS DATA DATA-ERR MISC 3310600800012 NO-DIM NO-DIM NO-DIM NO-DIM 3310600800013 89. 35.70 0.15 0.55 3310600800014 91. 36.50 0.15 0.72 3310600800015 92. 37.00 0.07 0.68 3310600800016 93. 37.45 0.11 0.64 3310600800017 94. 37.87 0.08 0.60 3310600800018 95. 38.20 0.05 0.60 3310600800019 97. 38.90 0.07 0.67 3310600800020 103. 41.45 0.11 0.65 3310600800021 105. 42.35 0.11 0.60 3310600800022 106. 42.75 0.09 0.58 3310600800023 108. 43.45 0.12 0.58 3310600800024 ENDDATA 13 0 3310600800025 ENDSUBENT 24 0 3310600899999 SUBENT 33106009 20181230 31883310600900001 BIB 4 6 3310600900002 REACTION (96-CM-244(N,F)MASS,,ZP,,SPA) 3310600900003 ANALYSIS Gaussian fitting without considering the even-odd 3310600900004 effect 3310600900005 STATUS (TABLE) Table 3 of Applied Rad. Isotopes, 127 (2017) 923310600900006 (DEP,33106005) Fractional cumulative yield 3310600900007 MISC-COL (MISC) Charge dispersion parameter 3310600900008 ENDBIB 6 0 3310600900009 NOCOMMON 0 0 3310600900010 DATA 4 12 3310600900011 MASS DATA DATA-ERR MISC 3310600900012 NO-DIM NO-DIM NO-DIM NO-DIM 3310600900013 89. 36.00 0.07 0.60 3310600900014 90. 36.40 0.07 0.60 3310600900015 91. 36.90 0.13 0.74 3310600900016 92. 37.40 0.11 0.70 3310600900017 93. 37.80 0.13 0.65 3310600900018 94. 38.10 0.07 0.60 3310600900019 95. 38.40 0.14 0.65 3310600900020 97. 39.30 0.11 0.70 3310600900021 103. 41.68 0.15 0.65 3310600900022 105. 42.47 0.13 0.65 3310600900023 108. 43.75 0.13 0.60 3310600900024 112. 45.30 0.12 0.63 3310600900025 ENDDATA 14 0 3310600900026 ENDSUBENT 25 0 3310600999999 ENDENTRY 9 0 3310699999999