SUBENT 23194001 20130511 22352319400100001 BIB 16 135 2319400100002 TITLE The Zr-93(n,gamma) reaction up to 8 keV neutron energy2319400100003 REFERENCE (J,PR/C,87,014622,2013) 2319400100004 #doi:10.1103/PhysRevC.87.014622 2319400100005 Main reference. 2319400100006 AUTHOR (G.Tagliente,P.M.Milazzo, K.Fujii,U.Abbondanno,G.Aerts,2319400100007 H.Alvarez, F.Alvarez-Velarde, S.Andriamonje, 2319400100008 J.Andrzejewski,L.Audouin,G.Badurek, P.Baumann,F.Becvar,2319400100009 F.Belloni, E.Berthoumieux, F.Calvino, M.Calviani, 2319400100010 D.Cano-Ott,R.Capote, C.Carrappico, P.Cennini, V.Chepel,2319400100011 E.Chiaveri, N.Colonna, G.Cortes, A.Couture, M.Dahlfors,2319400100012 S.David, I.Dillmann, C.Domingo-Pardo, W.Dridi, I.Duran,2319400100013 C.Eleftheriadis, M.Embid-Segura, A.Ferrari, 2319400100014 R.Ferreira-Marques, W.Furman, I.Goncalves, 2319400100015 E.Gonzalez-Romero, F.Gramegna, C.Guerrero, F.Gunsing, 2319400100016 B.Haas, R.Haight, M.Heil,A.Herrera-Martinez, E.Jericha,2319400100017 F.Kaeppeler, Y.Kadi,D.Karadimos,D.Karamanis, M.Kerveno,2319400100018 E.Kossionides, M.Krticka,C.Lamboudis, H.Leeb,A.Lindote,2319400100019 I.Lopes, S.Lukic, J.Marganiec, S.Marrone, T.Martinez, 2319400100020 C.Massimi, P.Mastinu, A.Mengoni, C.Moreau, M.Mosconi, 2319400100021 F.Neves, H.Oberhummer, S.O'Brien, C.Papachristodoulou, 2319400100022 C.Papadopoulos, C.Paradela, N.Patronis, A.Pavlik, 2319400100023 P.Pavlopoulos, L.Perrot, M.T.Pigni, R.Plag, A.Plompen, 2319400100024 A.Plukis,A.Poch,J.Praena,C.Pretel,J.Quesada,R.Reifarth,2319400100025 M.Rosetti, C.Rubbia, G.Rudolf, P.Rullhusen, J.Salgado, 2319400100026 C.Santos,L.Sarchiapone,I.Savvidis, C.Stephan, J.L.Tain,2319400100027 L.Tassan-Got, L.Tavora, R.Terlizzi, G.Vannini, P.Vaz, 2319400100028 A.Ventura, D.Villamarin, M.C.Vincente, V.Vlachoudis, 2319400100029 R.Vlastou, F.Voss, S.Walter, M.Wiescher, K.Wisshak) 2319400100030 INSTITUTE (2ZZZNTF) n TOF collaboration. 2319400100031 (2ZZZCER) P.Cennini,E.Chiaveri,M.Dahlfors,A.Ferrari, 2319400100032 A.Herrera-Martinez,Y.Kadi,L.Sarchiapone,V.Vlachoudis. 2319400100033 (2ZZZGEL) A.Plompen,P.Rullhusen. 2319400100034 (2ITYBAU) G.Tagliente,N.Colonna,S.Marrone,R.Terlizzi. 2319400100035 (2ITYTRI) P.M.Milazzo,K.Fujii,U.Abbondanno,F.Belloni, 2319400100036 C.Moreau. 2319400100037 (2FR SAC) G.Aerts,S.Andriamonje,E.Berthoumieux,W.Dridi,2319400100038 F.Gunsing,L.Perrot, A.Plukis. 2319400100039 (2SPNSAU) H.Alvarez,I.Duran,C.Paradela, 2319400100040 (2SPNPCM) F.Alvarez-Velarde,D.Cano-Ott,M.Embid-Segura, 2319400100041 E.Gonzalez-Romero,C.Guerrero,T.Martinez,D.Villamarin, 2319400100042 M.C.Vincente. 2319400100043 (3POLLOU) J.Andrzejewski,J.Marganiec, 2319400100044 (2GERKFK) L.Audouin,I.Dillmann,M.Heil,F.Kaeppeler, 2319400100045 M.Mosconi,R.Plag,F.Voss,S.Walter,K.Wisshak. 2319400100046 (2AUSATI) G.Badurek,E.Jericha,H.Leeb,H.Oberhummer, 2319400100047 M.T.Pigni. 2319400100048 (2FR STR) P.Baumann,S.David,M.Kerveno,S.Lukic,G.Rudolf.2319400100049 (3CZRCHU) F.Becvar,M.Krticka. 2319400100050 (2SPNUPC) F.Calvino,G.Cortes,A.Poch,C.Pretel. 2319400100051 (2ITYPAD) M.Calviani,F.Gramegna,P.Mastinu,J.Praena. 2319400100052 (3ZZZIAE) R.Capote,A.Mengoni. 2319400100053 (2SPNSEU) R.Capote,J.Quesada. 2319400100054 (2PRTLFE) C.Carrappico,I.Goncalves,J.Salgado,C.Santos, 2319400100055 L.Tavora,P.Vaz. 2319400100056 (2PRTPRT) LIP - Coimbra and Departamento de Fisica da 2319400100057 Universidade de Coimbra, Portugal. 2319400100058 V.Chepel,R.Ferreira-Marques,A.Lindote,I.Lopes,F.Neves. 2319400100059 (1USANOT) A.Couture,S.O'Brien,M.Wiescher. 2319400100060 (2GERGSI) I.Dillmann,C.Domingo-Pardo,M.Heil, 2319400100061 J.Marganiec,R.Plag,R.Reifarth. 2319400100062 (2SPNVAL) C.Domingo-Pardo,J.L.Tain. 2319400100063 (2GRCARU) C.Eleftheriadis,C.Lamboudis,I.Savvidis. 2319400100064 (4ZZZDUB) W.Furman. 2319400100065 (2FR GRA) B.Haas. 2319400100066 (1USALAS) R.Haight,R.Reifarth. 2319400100067 (2GRCIOA) D.Karadimos,D.Karamanis,C.Papachristodoulou, 2319400100068 N.Patronis. 2319400100069 (2GRCATH) E.Kossionides. 2319400100070 (2ITYUBO) C.Massimi,G.Vannini. 2319400100071 (2GERPTB) M.Mosconi. 2319400100072 (2GRCTUA) C.Papadopoulos,R.Vlastou. 2319400100073 (2AUSVIE) A.Pavlik. 2319400100074 (2FR FR ) Pole Universitaire Leonard de Vinci, 2319400100075 Paris La Defense, Paris, France . 2319400100076 P.Pavlopoulos. 2319400100077 (2ITYBOL) M.Rosetti,A.Ventura. 2319400100078 (2ITYPAV) C.Rubbia. 2319400100079 (2FR PAR) C.Stephan,L.Tassan-Got. 2319400100080 REL-REF (I,,C.Borcea+,J,NIM/A,513,(3),524,2003) 2319400100081 Facility details . 2319400100082 (M,,U.Abbondanno+,J,NIM/A,521,454,2004) 2319400100083 PHWT - pulse height weighting technique. 2319400100084 FACILITY (SYNCY,2ZZZCER) 20-GeV/c proton synchro-cyclotron, 2319400100085 n-TOF facility, CERN. Pulsed proton beam of high 2319400100086 intensity of 7.E+12 protons per bunch. 2319400100087 INC-SOURCE (SPALL) Spallation reaction of fast protons on the 2319400100088 massive lead target moderated in a surrounding 2319400100089 5.8 cm thick water cooling layer surrounding the lead2319400100090 target.Pulse width 6 ns. 2319400100091 INC-SPECT Neutron flux 10**5 neutrons/cm2/pulse at the sample 2319400100092 position). Resolution in neutron energy is better than 2319400100093 0.1% in the range of the present measurement, i.e. 2319400100094 below 8 keV. Nearly symmetrical Gaussian-shaped beam 2319400100095 profile at the sample position. 2319400100096 The neutron flux was determined relative to the 2319400100097 235U(n,f) cross section by means of calibrated fission 2319400100098 chamber from PTB Braunschweig. During the measurement 2319400100099 the flux was checked online by a low-mass 6Li neutron 2319400100100 monitor. 2319400100101 METHOD (TOF) Flight path 187.5 m from spallation target to 2319400100102 sample position. 2319400100103 PART-DET (G) Prompt gamma-ray cascade following neutron capture.2319400100104 DETECTOR (SCIN) Two C6-D6 liquid scintillator cells as gamma 2319400100105 detectors placed perpendicular to neutron beam at a 2319400100106 distance of about 3 cm from beam axis and 9.2 cm 2319400100107 backward from the sample position. Directly coupled 2319400100108 to EMI-9823QKB photomultiplier tubes. The light output 2319400100109 of the detectors was calibrated at 662, 1173, 1332 keV 2319400100110 by means of 137Cs and 60Co reference sources. An 2319400100111 additional calibration point at 6.13 MeV was obtained 2319400100112 by means of a composite 238Pu/13C source. 2319400100113 (FISCH,IOCH) U-235 loaded parallel-plate fission 2319400100114 chamber from PTB Braunschweig - for neutron flux 2319400100115 measurement as well as Li-6 neutron flux monitors. 2319400100116 MONITOR (92-U-235(N,F),,SIG) For the neutron flux. 2319400100117 SAMPLE Zr-O2 oxide powder pressed to pellet of 22 mm diameter,2319400100118 thickness 3.5mm, mass 4.46 g, encapsulated twice in 2319400100119 inner Al and a welded outer Ti container, both with 2319400100120 0.2 mm thick walls. 93Zr activity was 62.6 MBq. 2319400100121 Isotope composition: 2319400100122 Zr-90 - 2.29%, Zr-91 - 18.61%, Zr-92 - 18.95%, 2319400100123 Zr-93 - 19.98, Zr-94 - 20.50%, Zr-96 - 19.67%. 2319400100124 Traces of Mo and S were also present in the sample - 2319400100125 below 0.01 %, the contribution of these impurities to 2319400100126 the measured capture yield was not negligible. 2319400100127 Au and Pb samples of the same diameter were used for 2319400100128 repeated neutron flux measurements and background runs.2319400100129 ANALYSIS The intrinsic efficiency of C6D6 detectors was modified2319400100130 by the pulse height weighting technique (PHWT). 2319400100131 CORRECTION For the stable zirconium isotopes, sample impurities, 2319400100132 and the various backgrounds. 2319400100133 For the energy resolution of the neutron beam, for the 2319400100134 Doppler broadening of cross-section line shapes, for 2319400100135 self-shielding and neutron multiple scattering. 2319400100136 HISTORY (20101014C) M.M. 2319400100137 ENDBIB 135 0 2319400100138 NOCOMMON 0 0 2319400100139 ENDSUBENT 138 0 2319400199999 SUBENT 23194009 20130511 22352319400900001 BIB 5 12 2319400900002 REACTION (40-ZR-93(N,G)40-ZR-94,,SIG,,MXW) MACS 2319400900003 ANALYSIS Results for restricted energy range were complemented2319400900004 for the neutron energy range above 8 keV with Zr-93 c-s2319400900005 from JENDL-4.0 library. 2319400900006 REL-REF (A,V0102163,Z.Y.Bao+,J,AND,76,70,2000) 2319400900007 Agree with recommended value of Z.Bao+ at 30 keV - 2319400900008 95+-10 mb . 2319400900009 ERR-ANALYS (DATA-ERR) Error includes: 2319400900010 (DATA-ERR1) Uncertainty of present data ( < 8 keV) - 5%2319400900011 (ERR-2) Uncertainty of evaluated data above 8 keV - 10%2319400900012 STATUS (TABLE) Table I of J,PR/C,87,014622,2013 . 2319400900013 (DEP,23194008) MACS for energy <8 keV. 2319400900014 ENDBIB 12 0 2319400900015 COMMON 2 3 2319400900016 DATA-ERR1 ERR-2 2319400900017 PER-CENT PER-CENT 2319400900018 5. 10. 2319400900019 ENDCOMMON 3 0 2319400900020 DATA 3 6 2319400900021 KT DATA DATA-ERR 2319400900022 KEV MB MB 2319400900023 5. 347. 19. 2319400900024 10. 215. 17. 2319400900025 15. 160. 14. 2319400900026 20. 129. 12. 2319400900027 25. 110. 10. 2319400900028 30. 96. 9. 2319400900029 ENDDATA 8 0 2319400900030 ENDSUBENT 29 0 2319400999999